Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel Cathodes

Almodóvar, Paloma; Rey-Raap, Natalia; Flores López, Samantha Lizette; Sotillo, Belén; Santos, Lara; Tinoco, Miguel; Ramírez-Castellanos, Julio; Álvarez-Serrano, Inmaculada; López, María Luisa; Cameán Martínez, Ignacio; Arenillas de la Puente, Ana; Chacón, Joaquín; García Suárez, Ana Beatriz

Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel Cathodes

This study presents groundbreaking results in the field of rechargeable aluminium-ion batteries, achieving stable capacities exceeding 300 mAh g−1 for more than 300 cycles. The key to this achievement lies in the utilization of tailor-made carbon materials and a urea-AlCl3-based electrolyte. The art...

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Autores:	Almodóvar, Paloma, Rey-Raap, Natalia, Flores López, Samantha Lizette, Sotillo, Belén, Santos, Lara, Tinoco, Miguel, Ramírez-Castellanos, Julio, Álvarez-Serrano, Inmaculada, López, María Luisa, Cameán Martínez, Ignacio, Arenillas de la Puente, Ana, Chacón, Joaquín, García Suárez, Ana Beatriz
Tipo de recurso:	artículo
Estado:	Versión aceptada para publicación
Fecha de publicación:	2024
País:	España
Institución:	Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:	DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:	oai:digital.csic.es:10261/383320
Acceso en línea:	http://hdl.handle.net/10261/383320 https://api.elsevier.com/content/abstract/scopus_id/85197151365
Access Level:	acceso abierto
Palabra clave:	rechargeable Al-ion battery carbon xerogel cathode nitrogen http://metadata.un.org/sdg/7 http://metadata.un.org/sdg/9 Ensure access to affordable, reliable, sustainable and modern energy for all Build resilient infrastructure, promote inclusive and sustainable industrialization and foster innovation

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spelling	Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel CathodesAlmodóvar, PalomaRey-Raap, NataliaFlores López, Samantha LizetteSotillo, BelénSantos, LaraTinoco, MiguelRamírez-Castellanos, JulioÁlvarez-Serrano, InmaculadaLópez, María LuisaCameán Martínez, IgnacioArenillas de la Puente, AnaChacón, JoaquínGarcía Suárez, Ana BeatrizrechargeableAl-ion batterycarbon xerogelcathodenitrogenhttp://metadata.un.org/sdg/7http://metadata.un.org/sdg/9Ensure access to affordable, reliable, sustainable and modern energy for allBuild resilient infrastructure, promote inclusive and sustainable industrialization and foster innovationThis study presents groundbreaking results in the field of rechargeable aluminium-ion batteries, achieving stable capacities exceeding 300 mAh g−1 for more than 300 cycles. The key to this achievement lies in the utilization of tailor-made carbon materials and a urea-AlCl3-based electrolyte. The article investigates the optimal physicochemical properties of the active material necessary for effective electrodes for these aluminium-ion batteries. This investigation employs a wide range of materials characterization techniques (XRD, SEM-EDX, N2 adsorption-desorption isotherms, Hg porosimetry, XPS, FTIR, Raman and TEM-EDX) and electrochemical performance analyses to delve into the subject. These findings represent a significant improvement in the capacity of aluminium-ion batteries, bringing us closer to their implementation and commercialization. This achievement is attributed to the utilization of readily available, cost-effective, and non-corrosive materials. The ability to customize carbon xerogels and the use of the urea-AlCl3 electrolyte offer promising avenues for the practical implementation of these advanced battery technologies, leading to further enhancements in their performance and widespread adoption in various applications.This research was funded by the Ministerio de Ciencia e Innovación de España, the European Union Next Generation EU/PRTR and Science, Technology and Innovation Plan2018–2022 of the Principado de Asturias with the projects PCI2020-112039 MCIN/ AEI-10.13039/501100011033, PID2020-113001RB-I00 MCIN/AEI- 10.13039/501100011033 and IDI/2021/50921. N. R.-R. is grateful to the Horizon-MSCA-2021-PF-01-01 call for financial support through the Metgel project 101059852.Peer reviewedJohn Wiley & SonsMinisterio de Ciencia e Innovación (España)Principado de AsturiasEuropean CommissionRey-Raap, Natalia [0000-0002-5003-0035]Flores López, Samantha Lizette [0000-0002-6954-2348]Arenillas de la Puente, Ana [0000-0002-5388-1169]Cameán Martínez, Ignacio [0000-0003-4014-0385]García Suárez, Ana Beatriz [0000-0003-0935-334X]Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]202520252024info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501Postprintinfo:eu-repo/semantics/acceptedVersionhttp://hdl.handle.net/10261/383320https://api.elsevier.com/content/abstract/scopus_id/85197151365reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Inglés#PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE#info:eu-repo/grantAgreement/MCIN//PCI2020-112039info:eu-repo/grantAgreement/MCIN//PID2020-113001RB-I00info:eu-repo/grantAgreement/MCIN//IDIinfo:eu-repo/grantAgreement/EC/HE/101059852Batteries and SupercapsSíinfo:eu-repo/semantics/openAccessoai:digital.csic.es:10261/3833202026-05-22T06:33:51Z
dc.title.none.fl_str_mv	Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel Cathodes
title	Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel Cathodes
spellingShingle	Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel Cathodes Almodóvar, Paloma rechargeable Al-ion battery carbon xerogel cathode nitrogen http://metadata.un.org/sdg/7 http://metadata.un.org/sdg/9 Ensure access to affordable, reliable, sustainable and modern energy for all Build resilient infrastructure, promote inclusive and sustainable industrialization and foster innovation
title_short	Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel Cathodes
title_full	Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel Cathodes
title_fullStr	Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel Cathodes
title_full_unstemmed	Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel Cathodes
title_sort	Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel Cathodes
dc.creator.none.fl_str_mv	Almodóvar, Paloma Rey-Raap, Natalia Flores López, Samantha Lizette Sotillo, Belén Santos, Lara Tinoco, Miguel Ramírez-Castellanos, Julio Álvarez-Serrano, Inmaculada López, María Luisa Cameán Martínez, Ignacio Arenillas de la Puente, Ana Chacón, Joaquín García Suárez, Ana Beatriz
author	Almodóvar, Paloma
author_facet	Almodóvar, Paloma Rey-Raap, Natalia Flores López, Samantha Lizette Sotillo, Belén Santos, Lara Tinoco, Miguel Ramírez-Castellanos, Julio Álvarez-Serrano, Inmaculada López, María Luisa Cameán Martínez, Ignacio Arenillas de la Puente, Ana Chacón, Joaquín García Suárez, Ana Beatriz
author_role	author
author2	Rey-Raap, Natalia Flores López, Samantha Lizette Sotillo, Belén Santos, Lara Tinoco, Miguel Ramírez-Castellanos, Julio Álvarez-Serrano, Inmaculada López, María Luisa Cameán Martínez, Ignacio Arenillas de la Puente, Ana Chacón, Joaquín García Suárez, Ana Beatriz
author2_role	author author author author author author author author author author author author
dc.contributor.none.fl_str_mv	Ministerio de Ciencia e Innovación (España) Principado de Asturias European Commission Rey-Raap, Natalia [0000-0002-5003-0035] Flores López, Samantha Lizette [0000-0002-6954-2348] Arenillas de la Puente, Ana [0000-0002-5388-1169] Cameán Martínez, Ignacio [0000-0003-4014-0385] García Suárez, Ana Beatriz [0000-0003-0935-334X] Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]
dc.subject.none.fl_str_mv	rechargeable Al-ion battery carbon xerogel cathode nitrogen http://metadata.un.org/sdg/7 http://metadata.un.org/sdg/9 Ensure access to affordable, reliable, sustainable and modern energy for all Build resilient infrastructure, promote inclusive and sustainable industrialization and foster innovation
topic	rechargeable Al-ion battery carbon xerogel cathode nitrogen http://metadata.un.org/sdg/7 http://metadata.un.org/sdg/9 Ensure access to affordable, reliable, sustainable and modern energy for all Build resilient infrastructure, promote inclusive and sustainable industrialization and foster innovation
description	This study presents groundbreaking results in the field of rechargeable aluminium-ion batteries, achieving stable capacities exceeding 300 mAh g−1 for more than 300 cycles. The key to this achievement lies in the utilization of tailor-made carbon materials and a urea-AlCl3-based electrolyte. The article investigates the optimal physicochemical properties of the active material necessary for effective electrodes for these aluminium-ion batteries. This investigation employs a wide range of materials characterization techniques (XRD, SEM-EDX, N2 adsorption-desorption isotherms, Hg porosimetry, XPS, FTIR, Raman and TEM-EDX) and electrochemical performance analyses to delve into the subject. These findings represent a significant improvement in the capacity of aluminium-ion batteries, bringing us closer to their implementation and commercialization. This achievement is attributed to the utilization of readily available, cost-effective, and non-corrosive materials. The ability to customize carbon xerogels and the use of the urea-AlCl3 electrolyte offer promising avenues for the practical implementation of these advanced battery technologies, leading to further enhancements in their performance and widespread adoption in various applications.
publishDate	2024
dc.date.none.fl_str_mv	2024 2025 2025
dc.type.none.fl_str_mv	info:eu-repo/semantics/article http://purl.org/coar/resource_type/c_6501 Postprint info:eu-repo/semantics/acceptedVersion
format	article
status_str	acceptedVersion
dc.identifier.none.fl_str_mv	http://hdl.handle.net/10261/383320 https://api.elsevier.com/content/abstract/scopus_id/85197151365
url	http://hdl.handle.net/10261/383320 https://api.elsevier.com/content/abstract/scopus_id/85197151365
dc.language.none.fl_str_mv	Inglés
language_invalid_str_mv	Inglés
dc.relation.none.fl_str_mv	#PLACEHOLDER_PARENT_METADATA_VALUE# #PLACEHOLDER_PARENT_METADATA_VALUE# #PLACEHOLDER_PARENT_METADATA_VALUE# #PLACEHOLDER_PARENT_METADATA_VALUE# info:eu-repo/grantAgreement/MCIN//PCI2020-112039 info:eu-repo/grantAgreement/MCIN//PID2020-113001RB-I00 info:eu-repo/grantAgreement/MCIN//IDI info:eu-repo/grantAgreement/EC/HE/101059852 Batteries and Supercaps Sí
dc.rights.none.fl_str_mv	info:eu-repo/semantics/openAccess
eu_rights_str_mv	openAccess
dc.publisher.none.fl_str_mv	John Wiley & Sons
publisher.none.fl_str_mv	John Wiley & Sons
dc.source.none.fl_str_mv	reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str	Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str	DIGITAL.CSIC. Repositorio Institucional del CSIC
collection	DIGITAL.CSIC. Repositorio Institucional del CSIC
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repository.mail.fl_str_mv
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score	15,811543

Enhancing Aluminium-Ion Battery Performance with Carbon Xerogel Cathodes

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