Neodymium recovery from the aqueous phase using a residual material from saccharified banana-rachis/polyethylene-glycol

Neodymium (Nd) is a key rare earth element (REE) needed for the future of incoming technologies including road transport and power generation. Hereby, a sustainable adsorbent material for recovering Nd from the aqueous phase using a residue from the saccharification process is presented. Banana rach...

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Detalles Bibliográficos
Autores: Lapo Calderón, Byron Gonzalo, Pavón Regaña, Sandra|||0000-0002-6577-386X, Bertau, Martin, Demey Cedeño, Hary, Meneses, Miguel, Sastre Requena, Ana María|||0000-0002-6586-8113
Tipo de recurso: artículo
Fecha de publicación:2023
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/387305
Acceso en línea:https://hdl.handle.net/2117/387305
https://dx.doi.org/10.3390/polym15071666
Access Level:acceso abierto
Palabra clave:Neodymium
Rare earth recovery
Sorption
Lignocellulosic waste
PEG
Neodimi
Àrees temàtiques de la UPC::Enginyeria química
Descripción
Sumario:Neodymium (Nd) is a key rare earth element (REE) needed for the future of incoming technologies including road transport and power generation. Hereby, a sustainable adsorbent material for recovering Nd from the aqueous phase using a residue from the saccharification process is presented. Banana rachis (BR) was treated with cellulases and polyethylene glycol (PEG) to produce fermentable sugars prior to applying the final residue (BR–PEG) as an adsorbent material. BR–PEG was characterized by scanning electron microscopy (SEM), compositional analysis, pH of zero charge (pHpzc), Fourier transform infrared analysis (FTIR) and thermogravimetric analysis (TGA). A surface response experimental design was used for obtaining the optimized adsorption conditions in terms of the pH of the aqueous phase and the particle size. With the optimal conditions, equilibrium isotherms, kinetics and adsorption–desorption cycles were performed. The optimal pH and particle size were 4.5 and 209.19 µm, respectively. BR–PEG presented equilibrium kinetics after 20 min and maximum adsorption capacities of 44.11 mg/g. In terms of reusage, BR–PEG can be efficiently reused for five adsorption–desorption cycles. BR–PEG was demonstrated to be a low-cost bioresourced alternative for recovering Nd by adsorption.