Nanogold mesoporous iron promoted ceria catalysts for total and preferential CO oxidation reactions

Herein, a series of highly efficient gold based catalysts supported on mesoporous CeO2-Fe2O3 mixed oxides for CO elimination reactions have been developed. The materials have been fully characterized by means of XRD, Raman and UV-Vis spectroscopies among other techniques. We identify the Ce-Fe syner...

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Detalles Bibliográficos
Autores: Ramírez-Reina, Tomás, Ivanova, Svetlana, Idakiev, Vasko, Tabakova, Tatiana, Centeno, Miguel Ángel, Deng, Qing-Fang, Yuan, Zhong-Yong, Odriozola, José Antonio
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2016
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/127835
Acceso en línea:http://hdl.handle.net/10261/127835
Access Level:acceso abierto
Palabra clave:Gold catalysts
Mesoporous cerium oxide
Low temperature
CO oxidation
PrOx
H2 purification.
Descripción
Sumario:Herein, a series of highly efficient gold based catalysts supported on mesoporous CeO2-Fe2O3 mixed oxides for CO elimination reactions have been developed. The materials have been fully characterized by means of XRD, Raman and UV-Vis spectroscopies among other techniques. We identify the Ce-Fe synergism as a fundamental factor controlling the catalytic performance. Our data clearly reveal that the CO oxidation activity is maximized when the electronic and structural properties of the support are carefully controlled. In this situation, fairly good catalysts for environmental applications as for example H2 streams purification for fuel cell goals or CO abatement at room temperature can be designed