Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes [Dataset]

[Description of methods used for collection/generation of data] Data acquired with a high-kinetic-energy Scienta EW 4000 hemispherical analyser installed on the HAXPES endstation of the GALAXIES beamline of the French national synchrotron facility SOLEIL (France) [Methods for processing the data] Ca...

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Autores: Capone, F., Muntada, Olga, Ramírez, Jéssica Casandra, Esplandiú, María J., Dedryvère, R., Grimaud, A., Lassalle-Kaiser, B., Céolin, D., Perez Murano, Francesc X., Rueff, J. P., Fraxedas, J.
Tipo de recurso: conjunto de datos
Fecha de publicación:2024
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/369887
Acceso en línea:http://hdl.handle.net/10261/369887
https://doi.org/10.20350/digitalCSIC/16611
Access Level:acceso abierto
Palabra clave:Hard X-ray photoelectron spectroscopy (HAXPES)
Photoemission of liquids
Synchrotron radiation
Silicon nitride membranes
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oai_identifier_str oai:digital.csic.es:10261/369887
network_acronym_str ES
network_name_str España
repository_id_str
dc.title.none.fl_str_mv Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes [Dataset]
title Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes [Dataset]
spellingShingle Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes [Dataset]
Capone, F.
Hard X-ray photoelectron spectroscopy (HAXPES)
Photoemission of liquids
Synchrotron radiation
Silicon nitride membranes
title_short Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes [Dataset]
title_full Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes [Dataset]
title_fullStr Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes [Dataset]
title_full_unstemmed Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes [Dataset]
title_sort Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes [Dataset]
dc.creator.none.fl_str_mv Capone, F.
Muntada, Olga
Ramírez, Jéssica Casandra
Esplandiú, María J.
Dedryvère, R.
Grimaud, A.
Lassalle-Kaiser, B.
Céolin, D.
Perez Murano, Francesc X.
Rueff, J. P.
Fraxedas, J.
author Capone, F.
author_facet Capone, F.
Muntada, Olga
Ramírez, Jéssica Casandra
Esplandiú, María J.
Dedryvère, R.
Grimaud, A.
Lassalle-Kaiser, B.
Céolin, D.
Perez Murano, Francesc X.
Rueff, J. P.
Fraxedas, J.
author_role author
author2 Muntada, Olga
Ramírez, Jéssica Casandra
Esplandiú, María J.
Dedryvère, R.
Grimaud, A.
Lassalle-Kaiser, B.
Céolin, D.
Perez Murano, Francesc X.
Rueff, J. P.
Fraxedas, J.
author2_role author
author
author
author
author
author
author
author
author
author
dc.contributor.none.fl_str_mv European Commission
Ministerio de Ciencia e Innovación (España)
Agencia Estatal de Investigación (España)
Generalitat de Catalunya
Fraxedas, J. [0000-0002-2821-4831]
Esplandiú, María J. [0000-0003-2079-0639]
Perez Murano, Francesc X. [0000-0002-4647-8558]
Ramírez, Jéssica Casandra [0000-0003-2529-807X]
Fraxedas, J. [jordi.fraxedas@icn2.cat]
Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]
dc.subject.none.fl_str_mv Hard X-ray photoelectron spectroscopy (HAXPES)
Photoemission of liquids
Synchrotron radiation
Silicon nitride membranes
topic Hard X-ray photoelectron spectroscopy (HAXPES)
Photoemission of liquids
Synchrotron radiation
Silicon nitride membranes
description [Description of methods used for collection/generation of data] Data acquired with a high-kinetic-energy Scienta EW 4000 hemispherical analyser installed on the HAXPES endstation of the GALAXIES beamline of the French national synchrotron facility SOLEIL (France) [Methods for processing the data] CasaXPS software.
publishDate 2024
dc.date.none.fl_str_mv 2024
2024
2024
dc.type.none.fl_str_mv info:eu-repo/semantics/dataset
http://purl.org/coar/resource_type/c_ddb1
format dataset
dc.identifier.none.fl_str_mv http://hdl.handle.net/10261/369887
https://doi.org/10.20350/digitalCSIC/16611
url http://hdl.handle.net/10261/369887
https://doi.org/10.20350/digitalCSIC/16611
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
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info:eu-repo/grantAgreement/EC/H2020/101007417
info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/PID2021-124568NB-I00
info:eu-repo/grantAgreement/EC/H2020/957189
info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/CEX2021-001214-S
info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/CEX2023-001397-M
Capone, F.; Muntada, Olga; Ramírez, Jhonattan C.; Esplandiú, María J.; Dedryvère, R.; Grimaud, A.; Lassalle-Kaiser, B.; Céolin, D.; Perez Murano, Francesc X.; Rueff, J. P.; Fraxedas, J. Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes. https://doi.org/10.1107/S1600577524008865 . http://hdl.handle.net/10261/369707
CasaXPS software
Sí
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/vnd.ms-excel
dc.publisher.none.fl_str_mv DIGITAL.CSIC
publisher.none.fl_str_mv DIGITAL.CSIC
dc.source.none.fl_str_mv reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC
instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str DIGITAL.CSIC. Repositorio Institucional del CSIC
collection DIGITAL.CSIC. Repositorio Institucional del CSIC
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spelling Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes [Dataset]Capone, F.Muntada, OlgaRamírez, Jéssica CasandraEsplandiú, María J.Dedryvère, R.Grimaud, A.Lassalle-Kaiser, B.Céolin, D.Perez Murano, Francesc X.Rueff, J. P.Fraxedas, J.Hard X-ray photoelectron spectroscopy (HAXPES)Photoemission of liquidsSynchrotron radiationSilicon nitride membranes[Description of methods used for collection/generation of data] Data acquired with a high-kinetic-energy Scienta EW 4000 hemispherical analyser installed on the HAXPES endstation of the GALAXIES beamline of the French national synchrotron facility SOLEIL (France) [Methods for processing the data] CasaXPS software.Original raw data (uncorrected energies) of HAXPES spectra obtained at the HAXPES endstation of the GALAXIES beamline at SOLEIL synchrotron facility (France). Each spectrum is displayed in a two-column format, kinetic energy (X) vs. HAXPES intensity (Y). Photon energies are indicated for each figure.[FIGURE 5] HAXPES raw data of the Au 4f region in kinetic energy (X) vs. intensity (Y) columns of a 40 nm Au film (au_film_40nm), a dispersion of Au nanoparticles on a 25 nm-thick membrane in air (au_np_cell16), a dispersion of Au nanoparticles in MilliQ water (au_np_cell17) and a Au film treated with oxygen plasma and measured with 1486.6 eV photons (au_film_O2_plasma, data from DOI: 10.1021/acs.accounts.8b00241). Photon energy = 5 keV.[FIGURE 6] HAXPES raw and normalized (norm) data of the (a) N 1s, (b) O 1s, (c) C 1s and (d) F 1s lines obtained with 7 keV photons and using 20 nm thick membranes. Liquid cells filled with: air (S2), vacuum (S4), with air and with a ca 5 nm-thick amorphous carbon coating deposited in the inner part of the membrane (S7) and with 60 ml of the LP57 electrolyte (1 M LiPF6 in EC:EMC 3:7) and with the ca 5 nm-thick carbon coating (S6). The formulas used for normalization (heights normalized to their corresponding maxima) are displayed in the corresponding Y columns. In Fig. 6(d) a least-squares fit using the CasaXPS software after a Shirley-type background subtraction using a combination of Gaussian (70%) and Lorentzian (30%) functions under the constraint of identical full width at half-maximum (FWHM) for all components is shown. Raw and corrected kinetic energies are given.[FIGURE 7] HAXPES raw data of the (a) Na 1s region of a 3.5 M NaCl aqueous solution and (b) Cs 3d and (c) Cs 4d lines of a 2.6 M aqueous solution of CsCl obtained with 7 keV photons and using 15 nm membranes.[FIGURE S1] (Top) simulation of the inelastic mean free path (nm) as a function of the kinetic energy in silicon nitride using the TPP-2M model and assuming a 3.44 gr cm-3 density for silicon nitride. (Bottom) Simulated HAXPES spectra assuming a 15 nm thick silicon nitride layer on a CsCl substrate in the 3-10 keV photon energy range.European Union’s Horizon 2020 research and innovation programme, under grant agreement No. 101007417 NFFA-Europe Pilot. Spanish Ministry of Science and Innovation (MCIN) under contract No. PID2021-124568NB-I00. ICN2 is funded by the CERCA program/Generalitat de Catalunya. ICN2 is supported by the Severo Ochoa Centres of Excellence programme, grant CEX2021-001214-S, funded by MCIN/AEI. Support through the Marıa de Maeztu grant CEX2023-001397-M funded by MICIU/AEI is acknowledged. Generalitat de Catalunya through the 2021-SGR-00644 project. European Union’s Horizon 2020 research and innovation programme under grant agreement No. 957189.With funding from the Spanish government through the "Severo Ochoa Centre of Excellence" accreditation (CEX2021-001214-S).With funding from the Spanish government through the "Severo Ochoa Centre of Excellence" accreditation (CEX2023-001397-M).File List: Fig_5.xls; Fig_6a.xls, Fig_6b.xls, Fig_6c.xls, Fig_6d.xls, Fig_7.xls, Fig_S1.xlsPeer reviewedDIGITAL.CSICEuropean CommissionMinisterio de Ciencia e Innovación (España)Agencia Estatal de Investigación (España)Generalitat de CatalunyaFraxedas, J. [0000-0002-2821-4831]Esplandiú, María J. [0000-0003-2079-0639]Perez Murano, Francesc X. [0000-0002-4647-8558]Ramírez, Jéssica Casandra [0000-0003-2529-807X]Fraxedas, J. [jordi.fraxedas@icn2.cat]Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]202420242024info:eu-repo/semantics/datasethttp://purl.org/coar/resource_type/c_ddb1application/vnd.ms-excelhttp://hdl.handle.net/10261/369887https://doi.org/10.20350/digitalCSIC/16611reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Inglés#PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE#info:eu-repo/grantAgreement/EC/H2020/101007417info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/PID2021-124568NB-I00info:eu-repo/grantAgreement/EC/H2020/957189info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/CEX2021-001214-Sinfo:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/CEX2023-001397-MCapone, F.; Muntada, Olga; Ramírez, Jhonattan C.; Esplandiú, María J.; Dedryvère, R.; Grimaud, A.; Lassalle-Kaiser, B.; Céolin, D.; Perez Murano, Francesc X.; Rueff, J. P.; Fraxedas, J. Development of hard X-ray photoelectron spectroscopy in liquid cells using optimized microfabricated silicon nitride membranes. https://doi.org/10.1107/S1600577524008865 . http://hdl.handle.net/10261/369707CasaXPS softwareSíinfo:eu-repo/semantics/openAccessoai:digital.csic.es:10261/3698872026-05-22T06:33:51Z
score 15,81155

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