Connecting C≡C bonds to tetrairidium chains

The chain gang! Tetrametallic iridium chains with the metal atoms in an average oxidation state 1.5 and bound by unsupported metal-metal bonds have been effectively connected to organic fragments with delocalized π electrons, such as 1,4-diethynylbenzene (see figure). This connection allows an elect...

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Autores: Río, M. Pilar del, López, José A., Ciriano, Miguel A., Tejel, Cristina
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2013
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/108429
Acceso en línea:http://hdl.handle.net/10261/108429
Access Level:acceso abierto
Palabra clave:Metal–metal interactions
Electronic delocalization
Iridium
Acetylides
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spelling Connecting C≡C bonds to tetrairidium chainsRío, M. Pilar delLópez, José A.Ciriano, Miguel A.Tejel, CristinaMetal–metal interactionsElectronic delocalizationIridiumAcetylidesThe chain gang! Tetrametallic iridium chains with the metal atoms in an average oxidation state 1.5 and bound by unsupported metal-metal bonds have been effectively connected to organic fragments with delocalized π electrons, such as 1,4-diethynylbenzene (see figure). This connection allows an electronic communication along the whole chain spanning around 30 Å and sheds light on the possible use of this type of molecule as "molecular wires". Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.Funded by: MICINN/FEDER. Grant Number: CTQ2011-22516 and Gobierno de Aragón (GA)/FSE (E70).Peer ReviewedWiley-VCHGobierno de AragónMinisterio de Ciencia e Innovación (España)European Commission2014201420132014info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501Postprintinfo:eu-repo/semantics/acceptedVersionhttp://hdl.handle.net/10261/108429reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Ingléshttp://dx.doi.org/10.1002/chem.201203769info:eu-repo/semantics/openAccessoai:digital.csic.es:10261/1084292026-05-22T06:33:51Z
dc.title.none.fl_str_mv Connecting C≡C bonds to tetrairidium chains
title Connecting C≡C bonds to tetrairidium chains
spellingShingle Connecting C≡C bonds to tetrairidium chains
Río, M. Pilar del
Metal–metal interactions
Electronic delocalization
Iridium
Acetylides
title_short Connecting C≡C bonds to tetrairidium chains
title_full Connecting C≡C bonds to tetrairidium chains
title_fullStr Connecting C≡C bonds to tetrairidium chains
title_full_unstemmed Connecting C≡C bonds to tetrairidium chains
title_sort Connecting C≡C bonds to tetrairidium chains
dc.creator.none.fl_str_mv Río, M. Pilar del
López, José A.
Ciriano, Miguel A.
Tejel, Cristina
author Río, M. Pilar del
author_facet Río, M. Pilar del
López, José A.
Ciriano, Miguel A.
Tejel, Cristina
author_role author
author2 López, José A.
Ciriano, Miguel A.
Tejel, Cristina
author2_role author
author
author
dc.contributor.none.fl_str_mv Gobierno de Aragón
Ministerio de Ciencia e Innovación (España)
European Commission
dc.subject.none.fl_str_mv Metal–metal interactions
Electronic delocalization
Iridium
Acetylides
topic Metal–metal interactions
Electronic delocalization
Iridium
Acetylides
description The chain gang! Tetrametallic iridium chains with the metal atoms in an average oxidation state 1.5 and bound by unsupported metal-metal bonds have been effectively connected to organic fragments with delocalized π electrons, such as 1,4-diethynylbenzene (see figure). This connection allows an electronic communication along the whole chain spanning around 30 Å and sheds light on the possible use of this type of molecule as "molecular wires". Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
publishDate 2013
dc.date.none.fl_str_mv 2013
2014
2014
2014
dc.type.none.fl_str_mv info:eu-repo/semantics/article
http://purl.org/coar/resource_type/c_6501
Postprint
info:eu-repo/semantics/acceptedVersion
format article
status_str acceptedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/10261/108429
url http://hdl.handle.net/10261/108429
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv http://dx.doi.org/10.1002/chem.201203769
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.publisher.none.fl_str_mv Wiley-VCH
publisher.none.fl_str_mv Wiley-VCH
dc.source.none.fl_str_mv reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC
instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str DIGITAL.CSIC. Repositorio Institucional del CSIC
collection DIGITAL.CSIC. Repositorio Institucional del CSIC
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