Removal of oxyfluorfen from polluted effluents by combined bio-electro processes

In this work, the combination of biological and electrochemical processes to mineralize oxyfluorfen has been studied. First, an acclimatized mixed-culture biological treatment was used to degrade the biodegradable fraction of the pesticide, reaching up to 90% removal. After that, the non-biodegraded...

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Detalhes bibliográficos
Autores: Carboneras Contreras, María Belén, Rodrigo Rodrigo, Manuel Andrés, Cañizares Cañizares, Pablo, Villaseñor Camacho, José, Fernández Morales, Francisco Jesús
Tipo de documento: artigo
Data de publicação:2020
País:España
Recursos:Universidad de Castilla-La Mancha
Repositório:RUIdeRA. Repositorio Institucional de la UCLM
OAI Identifier:oai:ruidera.uclm.es:10578/29212
Acesso em linha:http://hdl.handle.net/10578/29212
Access Level:Acceso aberto
Palavra-chave:Ingeniería Química
Herbicida
Tratamiento biológico
Tratamiento electroquímico
Proceso combinado
Diamante dopado con boro
Descrição
Resumo:In this work, the combination of biological and electrochemical processes to mineralize oxyfluorfen has been studied. First, an acclimatized mixed-culture biological treatment was used to degrade the biodegradable fraction of the pesticide, reaching up to 90% removal. After that, the non-biodegraded fraction was oxidised by electrolysis using boron-doped diamond as the anode. The results showed that the electrochemical technique was able to completely mineralize the residual pollutants. The study of the influence of the supporting electrolyte on the electrochemical process showed that the trace mineral solution used in the biological treatment was enough to completely mineralize the oxyfluorfen, resulting in total organic carbon removal rates that were well-fitted by a first-order model with a kinetic constant of 0.91 h−1. However, the first-order degradation rate increased approximately 20% when Na2SO4 was added as supporting electrolyte, reaching a degradation rate of 1.16 h−1 with a power consumption that was approximately 70% lower.