Synthesis of Cobalt-Based Nanoparticles as Catalysts for Methanol Synthesis from CO2 Hydrogenation

The increasing emission of carbon dioxide into the atmosphere has urged the scientific community to investigate alternatives to alleviate such emissions, being that they are the principal contributor to the greenhouse gas effect. One major alternative is carbon capture and utilization (CCU) toward t...

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Autores: Carrasco García, Anna|||0000-0001-6215-5364, Vali, Seyed Alireza|||0000-0002-0124-9321, Ben-Abbou, Zahra, Moral-Vico, Javier|||0000-0002-6795-3450, Abo Markeb, Ahmad|||0000-0003-4385-0198, Sánchez, Antoni|||0000-0003-4254-8528
Formato: artículo
Fecha de publicación:2024
País:España
Recursos:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:289323
Acesso em linha:https://ddd.uab.cat/record/289323
https://dx.doi.org/urn:doi:10.3390/ma17030697
Access Level:acceso abierto
Palavra-chave:Carbon dioxide hydrogenation
Methanol synthesis
Nanomaterials
Heterogeneous catalysis
Metal-support interaction
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spelling Synthesis of Cobalt-Based Nanoparticles as Catalysts for Methanol Synthesis from CO2 HydrogenationCarrasco García, Anna|||0000-0001-6215-5364Vali, Seyed Alireza|||0000-0002-0124-9321Ben-Abbou, ZahraMoral-Vico, Javier|||0000-0002-6795-3450Abo Markeb, Ahmad|||0000-0003-4385-0198Sánchez, Antoni|||0000-0003-4254-8528Carbon dioxide hydrogenationMethanol synthesisNanomaterialsHeterogeneous catalysisMetal-support interactionThe increasing emission of carbon dioxide into the atmosphere has urged the scientific community to investigate alternatives to alleviate such emissions, being that they are the principal contributor to the greenhouse gas effect. One major alternative is carbon capture and utilization (CCU) toward the production of value-added chemicals using diverse technologies. This work aims at the study of the catalytic potential of different cobalt-derived nanoparticles for methanol synthesis from carbon dioxide hydrogenation. Thanks to its abundance and cost efficacy, cobalt can serve as an economical catalyst compared to noble metal-based catalysts. In this work, we present a systematic comparison among different cobalt and cobalt oxide nanocomposites in terms of their efficiency as catalysts for carbon dioxide hydrogenation to methanol as well as how different supports, zeolites, MnO, and CeO, can enhance their catalytic capacity. The oxygen vacancies in the cerium oxide act as carbon dioxide adsorption and activation sites, which facilitates a higher methanol production yield. 22024-01-0120242024-01-01Articlehttp://purl.org/coar/resource_type/c_6501VoRhttp://purl.org/coar/version/c_970fb48d4fbd8a85info:eu-repo/semantics/articleapplication/pdfhttps://ddd.uab.cat/record/289323https://dx.doi.org/urn:doi:10.3390/ma17030697reponame:Dipòsit Digital de Documents de la UABinstname:Universitat Autònoma de BarcelonaInglésengMinisterio de Ciencia e Innovación https://doi.org/10.13039/501100004837 TED2021-130407B-I00open accesshttp://purl.org/coar/access_right/c_abf2Aquest document està subjecte a una llicència d'ús Creative Commons. Es permet la reproducció total o parcial, la distribució, la comunicació pública de l'obra i la creació d'obres derivades, fins i tot amb finalitats comercials, sempre i quan es reconegui l'autoria de l'obra original.https://creativecommons.org/licenses/by/4.0/info:eu-repo/semantics/openAccessoai:ddd.uab.cat:2893232026-06-06T12:50:31Z
dc.title.none.fl_str_mv Synthesis of Cobalt-Based Nanoparticles as Catalysts for Methanol Synthesis from CO2 Hydrogenation
title Synthesis of Cobalt-Based Nanoparticles as Catalysts for Methanol Synthesis from CO2 Hydrogenation
spellingShingle Synthesis of Cobalt-Based Nanoparticles as Catalysts for Methanol Synthesis from CO2 Hydrogenation
Carrasco García, Anna|||0000-0001-6215-5364
Carbon dioxide hydrogenation
Methanol synthesis
Nanomaterials
Heterogeneous catalysis
Metal-support interaction
title_short Synthesis of Cobalt-Based Nanoparticles as Catalysts for Methanol Synthesis from CO2 Hydrogenation
title_full Synthesis of Cobalt-Based Nanoparticles as Catalysts for Methanol Synthesis from CO2 Hydrogenation
title_fullStr Synthesis of Cobalt-Based Nanoparticles as Catalysts for Methanol Synthesis from CO2 Hydrogenation
title_full_unstemmed Synthesis of Cobalt-Based Nanoparticles as Catalysts for Methanol Synthesis from CO2 Hydrogenation
title_sort Synthesis of Cobalt-Based Nanoparticles as Catalysts for Methanol Synthesis from CO2 Hydrogenation
dc.creator.none.fl_str_mv Carrasco García, Anna|||0000-0001-6215-5364
Vali, Seyed Alireza|||0000-0002-0124-9321
Ben-Abbou, Zahra
Moral-Vico, Javier|||0000-0002-6795-3450
Abo Markeb, Ahmad|||0000-0003-4385-0198
Sánchez, Antoni|||0000-0003-4254-8528
author Carrasco García, Anna|||0000-0001-6215-5364
author_facet Carrasco García, Anna|||0000-0001-6215-5364
Vali, Seyed Alireza|||0000-0002-0124-9321
Ben-Abbou, Zahra
Moral-Vico, Javier|||0000-0002-6795-3450
Abo Markeb, Ahmad|||0000-0003-4385-0198
Sánchez, Antoni|||0000-0003-4254-8528
author_role author
author2 Vali, Seyed Alireza|||0000-0002-0124-9321
Ben-Abbou, Zahra
Moral-Vico, Javier|||0000-0002-6795-3450
Abo Markeb, Ahmad|||0000-0003-4385-0198
Sánchez, Antoni|||0000-0003-4254-8528
author2_role author
author
author
author
author
dc.subject.none.fl_str_mv Carbon dioxide hydrogenation
Methanol synthesis
Nanomaterials
Heterogeneous catalysis
Metal-support interaction
topic Carbon dioxide hydrogenation
Methanol synthesis
Nanomaterials
Heterogeneous catalysis
Metal-support interaction
description The increasing emission of carbon dioxide into the atmosphere has urged the scientific community to investigate alternatives to alleviate such emissions, being that they are the principal contributor to the greenhouse gas effect. One major alternative is carbon capture and utilization (CCU) toward the production of value-added chemicals using diverse technologies. This work aims at the study of the catalytic potential of different cobalt-derived nanoparticles for methanol synthesis from carbon dioxide hydrogenation. Thanks to its abundance and cost efficacy, cobalt can serve as an economical catalyst compared to noble metal-based catalysts. In this work, we present a systematic comparison among different cobalt and cobalt oxide nanocomposites in terms of their efficiency as catalysts for carbon dioxide hydrogenation to methanol as well as how different supports, zeolites, MnO, and CeO, can enhance their catalytic capacity. The oxygen vacancies in the cerium oxide act as carbon dioxide adsorption and activation sites, which facilitates a higher methanol production yield.
publishDate 2024
dc.date.none.fl_str_mv 2
2024-01-01
2024
2024-01-01
dc.type.none.fl_str_mv Article
http://purl.org/coar/resource_type/c_6501
VoR
http://purl.org/coar/version/c_970fb48d4fbd8a85
dc.type.openaire.fl_str_mv info:eu-repo/semantics/article
format article
dc.identifier.none.fl_str_mv https://ddd.uab.cat/record/289323
https://dx.doi.org/urn:doi:10.3390/ma17030697
url https://ddd.uab.cat/record/289323
https://dx.doi.org/urn:doi:10.3390/ma17030697
dc.language.none.fl_str_mv Inglés
eng
language_invalid_str_mv Inglés
language eng
dc.relation.none.fl_str_mv Ministerio de Ciencia e Innovación https://doi.org/10.13039/501100004837 TED2021-130407B-I00
dc.rights.none.fl_str_mv open access
http://purl.org/coar/access_right/c_abf2
https://creativecommons.org/licenses/by/4.0/
dc.rights.openaire.fl_str_mv info:eu-repo/semantics/openAccess
rights_invalid_str_mv open access
http://purl.org/coar/access_right/c_abf2
https://creativecommons.org/licenses/by/4.0/
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
dc.source.none.fl_str_mv reponame:Dipòsit Digital de Documents de la UAB
instname:Universitat Autònoma de Barcelona
instname_str Universitat Autònoma de Barcelona
reponame_str Dipòsit Digital de Documents de la UAB
collection Dipòsit Digital de Documents de la UAB
repository.name.fl_str_mv
repository.mail.fl_str_mv
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score 15.301603

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