Thermodynamic stability of ß-phases in Zr-Nb alloys

We investigate the contribution of mixing enthalpy, configurational entropy, vibrational entropy, and electronic entropy towards the thermodynamic stability of ß-(Zr,Nb) phases, to explain discrepancies in experimental observation of irradiated Zr-Nb alloys. Mixing enthalpy, configurational entropy,...

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Detalles Bibliográficos
Autores: Tuli, Vidur, Burr, Patrick, Claisse, Antoine, Cazorla Silva, Claudio|||0000-0002-6501-4513
Tipo de recurso: artículo
Fecha de publicación:2023
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/405396
Acceso en línea:https://hdl.handle.net/2117/405396
https://dx.doi.org/10.1103/PhysRevMaterials.7.113607
Access Level:acceso abierto
Palabra clave:Thermodynamics
Molecular dynamics
Thermodynamics of mixing
Entropy
Ab initio molecular dynamics
Termodinàmica
Dinàmica molecular
Àrees temàtiques de la UPC::Física
Descripción
Sumario:We investigate the contribution of mixing enthalpy, configurational entropy, vibrational entropy, and electronic entropy towards the thermodynamic stability of ß-(Zr,Nb) phases, to explain discrepancies in experimental observation of irradiated Zr-Nb alloys. Mixing enthalpy, configurational entropy, and electronic free energy alone are insufficient to explain the relative stability of these phases. This emphasises the need for accurate determination of the vibrational free energy contributions, which we calculated using ab initio molecular dynamics. Including vibrational free energy contributions predicts ß-Zr decomposition in to HCP-Zr and ß-Nb at temperatures below ~880 K, in line with experimental observations. The relative energy difference between ß-Zr decomposition between 600 and 1200 K is small (<0.1 eV/atom) and may explain the wide range of apparently stable ß phases observed in neutron and proton irradiated Zr-Nb alloys. Other factors that may contribute towards the stability of these phases are also discussed.