Hollow Gold Nanoparticles Produced by Femtosecond Laser Irradiation
[EN] Metallic hollow nanoparticles exhibit interesting optical properties that can be controlled by geometrical parameters. Irradiation with femtosecond laser pulses has emerged recently as a valuable tool for reshaping and size modification of plasmonic metal nanoparticles, thereby enabling the syn...
| Autores: | , , , , , , , , , , |
|---|---|
| Tipo de recurso: | artículo |
| Fecha de publicación: | 2020 |
| País: | España |
| Institución: | Universitat Politècnica de València (UPV) |
| Repositorio: | RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia |
| Idioma: | inglés |
| OAI Identifier: | oai:riunet.upv.es:10251/178176 |
| Acceso en línea: | https://riunet.upv.es/handle/10251/178176 |
| Access Level: | acceso abierto |
| Palabra clave: | Hollow nanoparticles Localized surface plasmon resonance Femtosecond laser pulses MATEMATICA APLICADA FISICA APLICADA |
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| dc.title.none.fl_str_mv |
Hollow Gold Nanoparticles Produced by Femtosecond Laser Irradiation |
| title |
Hollow Gold Nanoparticles Produced by Femtosecond Laser Irradiation |
| spellingShingle |
Hollow Gold Nanoparticles Produced by Femtosecond Laser Irradiation Castro-Palacio, Juan Carlos|||0000-0002-0132-9989 Hollow nanoparticles Localized surface plasmon resonance Femtosecond laser pulses MATEMATICA APLICADA FISICA APLICADA |
| title_short |
Hollow Gold Nanoparticles Produced by Femtosecond Laser Irradiation |
| title_full |
Hollow Gold Nanoparticles Produced by Femtosecond Laser Irradiation |
| title_fullStr |
Hollow Gold Nanoparticles Produced by Femtosecond Laser Irradiation |
| title_full_unstemmed |
Hollow Gold Nanoparticles Produced by Femtosecond Laser Irradiation |
| title_sort |
Hollow Gold Nanoparticles Produced by Femtosecond Laser Irradiation |
| dc.creator.none.fl_str_mv |
Castro-Palacio, Juan Carlos|||0000-0002-0132-9989 Fernández de Córdoba, Pedro|||0000-0002-0347-7280 Ladutenko, Konstantin Prada, Alejandro Gonzalez-Rubio, Guillermo Diaz-Nunez, Pablo Guerrero-Martinez, Andres Kohanoff, Jorge Perlado, José Manuel Pena-Rodriguez, Ovidio Rivera, Antonio |
| author |
Castro-Palacio, Juan Carlos|||0000-0002-0132-9989 |
| author_facet |
Castro-Palacio, Juan Carlos|||0000-0002-0132-9989 Fernández de Córdoba, Pedro|||0000-0002-0347-7280 Ladutenko, Konstantin Prada, Alejandro Gonzalez-Rubio, Guillermo Diaz-Nunez, Pablo Guerrero-Martinez, Andres Kohanoff, Jorge Perlado, José Manuel Pena-Rodriguez, Ovidio Rivera, Antonio |
| author_role |
author |
| author2 |
Fernández de Córdoba, Pedro|||0000-0002-0347-7280 Ladutenko, Konstantin Prada, Alejandro Gonzalez-Rubio, Guillermo Diaz-Nunez, Pablo Guerrero-Martinez, Andres Kohanoff, Jorge Perlado, José Manuel Pena-Rodriguez, Ovidio Rivera, Antonio |
| author2_role |
author author author author author author author author author author |
| dc.contributor.none.fl_str_mv |
Departamento de Física Aplicada Departamento de Matemática Aplicada Escuela Técnica Superior de Ingeniería Aeroespacial y Diseño Industrial Instituto Universitario de Matemática Pura y Aplicada Escuela Técnica Superior de Ingeniería Industrial Centro de Tecnologías Físicas: Acústica, Materiales y Astrofísica Comunidad de Madrid EUROfusion Consortium Russian Science Foundation Agencia Estatal de Investigación Ministerio de Ciencia, Innovación y Universidades Fondo Nacional de Desarrollo Científico y Tecnológico, Chile Comisión Nacional de Investigación Científica y Tecnológica, Chile Repositorio Institucional de la Universitat Politècnica de València Riunet |
| dc.subject.none.fl_str_mv |
Hollow nanoparticles Localized surface plasmon resonance Femtosecond laser pulses MATEMATICA APLICADA FISICA APLICADA |
| topic |
Hollow nanoparticles Localized surface plasmon resonance Femtosecond laser pulses MATEMATICA APLICADA FISICA APLICADA |
| description |
[EN] Metallic hollow nanoparticles exhibit interesting optical properties that can be controlled by geometrical parameters. Irradiation with femtosecond laser pulses has emerged recently as a valuable tool for reshaping and size modification of plasmonic metal nanoparticles, thereby enabling the synthesis of nanostructures with unique morphologies. In this Letter, we use classical molecular dynamics simulations to investigate the solid-to-hollow conversion of gold nanoparticles upon femtosecond laser irradiation. Here, we suggest an efficient method for producing hollow nanoparticles under certain specific conditions, namely that the particles should be heated to a maximum temperature between 2500 and 3500 K, followed by a fast quenching to room temperature, with cooling rates lower than 120 ps. Therefore, we describe the experimental conditions for efficiently producing hollow nanoparticles, opening a broad range of possibilities for applications in key areas, such as energy storage and catalysis. |
| publishDate |
2020 |
| dc.date.none.fl_str_mv |
2020 2020-07-02 |
| dc.type.none.fl_str_mv |
journal article http://purl.org/coar/resource_type/c_6501 VoR http://purl.org/coar/version/c_970fb48d4fbd8a85 |
| dc.type.openaire.fl_str_mv |
info:eu-repo/semantics/article |
| format |
article |
| dc.identifier.none.fl_str_mv |
https://riunet.upv.es/handle/10251/178176 |
| url |
https://riunet.upv.es/handle/10251/178176 |
| dc.language.none.fl_str_mv |
Inglés eng |
| language_invalid_str_mv |
Inglés |
| language |
eng |
| dc.relation.none.fl_str_mv |
Agencia Estatal de Investigación http://dx.doi.org/10.13039/501100011033 Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016 MAT2017-86659-R DISEÑO DE NANOESTRUCTURAS PLASMONICAS COLOIDALES COMO AGENTES DE CONTRASTE MULTIMODALES PARA BIOIMAGEN Y DIAGNOSTICO Ministerio de Ciencia, Innovación y Universidades https://doi.org/10.13039/100014440 PGC2018-096444-B-I00 Agencia Estatal de Investigación http://dx.doi.org/10.13039/501100011033 Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020 RTI2018-095844-B-I00 NUEVOS VECTORES DE ACIDOS NUCLEICOS BASADOS EN MATRICES LIPIDICAS Y NANOPARTICULAS PLASMONICAS DE ORO PARA TERAPIA GENICA CONTRA EL CANCER EUROfusion Consortium EUROfusion Consortium ENR-IFE19.CCFE-01 Caja de Ahorros del Mediterráneo https://doi.org/10.13039/100012818 P2018%2FNMT-4389 Caja de Ahorros del Mediterráneo https://doi.org/10.13039/100012818 P2018%2FEMT-4437 Fondo Nacional de Desarrollo Científico y Tecnológico, Chile https://doi.org/10.13039/501100002850 3190123 Fondo Nacional de Desarrollo Científico y Tecnológico, Chile https://doi.org/10.13039/501100002850 11180557 Comisión Nacional de Investigación Científica y Tecnológica, Chile https://doi.org/10.13039/501100009068 FB-0807 Russian Science Foundation https://doi.org/10.13039/501100006769 19-19-00683 |
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open access http://purl.org/coar/access_right/c_abf2 Reserva de todos los derechos http://rightsstatements.org/vocab/InC/1.0/ |
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info:eu-repo/semantics/openAccess |
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open access http://purl.org/coar/access_right/c_abf2 Reserva de todos los derechos http://rightsstatements.org/vocab/InC/1.0/ |
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openAccess |
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application/pdf application/pdf |
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American Chemical Society |
| publisher.none.fl_str_mv |
American Chemical Society |
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reponame:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia instname:Universitat Politècnica de València (UPV) |
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Universitat Politècnica de València (UPV) |
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RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia |
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RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia |
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1869420344182308864 |
| spelling |
Hollow Gold Nanoparticles Produced by Femtosecond Laser IrradiationCastro-Palacio, Juan Carlos|||0000-0002-0132-9989Fernández de Córdoba, Pedro|||0000-0002-0347-7280Ladutenko, KonstantinPrada, AlejandroGonzalez-Rubio, GuillermoDiaz-Nunez, PabloGuerrero-Martinez, AndresKohanoff, JorgePerlado, José ManuelPena-Rodriguez, OvidioRivera, AntonioHollow nanoparticlesLocalized surface plasmon resonanceFemtosecond laser pulsesMATEMATICA APLICADAFISICA APLICADA[EN] Metallic hollow nanoparticles exhibit interesting optical properties that can be controlled by geometrical parameters. Irradiation with femtosecond laser pulses has emerged recently as a valuable tool for reshaping and size modification of plasmonic metal nanoparticles, thereby enabling the synthesis of nanostructures with unique morphologies. In this Letter, we use classical molecular dynamics simulations to investigate the solid-to-hollow conversion of gold nanoparticles upon femtosecond laser irradiation. Here, we suggest an efficient method for producing hollow nanoparticles under certain specific conditions, namely that the particles should be heated to a maximum temperature between 2500 and 3500 K, followed by a fast quenching to room temperature, with cooling rates lower than 120 ps. Therefore, we describe the experimental conditions for efficiently producing hollow nanoparticles, opening a broad range of possibilities for applications in key areas, such as energy storage and catalysis.This work has been funded by the Spanish Ministry of Science, Innovation and Universities (MICIU) (Grants RTI2018-095844-B-I00, PGC2018-096444-B-I00, and MAT2017-86659-R), the EUROfusion Consortium through Project ENR-IFE19.CCFE-01, and the Madrid Regional Government (Grants P2018/NMT-4389 and P2018/EMT-4437). A.P. is thankful for the support of FONDECYT under Grants 3190123 and 11180557, as well as from Financiamiento Basal para Centros Cientificos y Tecnologicos de Excelencia FB-0807. K.L. acknowledges the support of the Russian Science Foundation (Project 19-19-00683). The authors acknowledge the computer resources and technical assistance provided by the Centro de Supercomputacion y Visualizacion de Madrid (CeSViMa) and the supercomputing infrastructure of the NLHPC (ECM-02). This Letter is based upon work from COST Action TUMIEE (CA17126)American Chemical SocietyDepartamento de Física AplicadaDepartamento de Matemática AplicadaEscuela Técnica Superior de Ingeniería Aeroespacial y Diseño IndustrialInstituto Universitario de Matemática Pura y AplicadaEscuela Técnica Superior de Ingeniería IndustrialCentro de Tecnologías Físicas: Acústica, Materiales y AstrofísicaComunidad de MadridEUROfusion ConsortiumRussian Science FoundationAgencia Estatal de InvestigaciónMinisterio de Ciencia, Innovación y UniversidadesFondo Nacional de Desarrollo Científico y Tecnológico, ChileComisión Nacional de Investigación Científica y Tecnológica, ChileRepositorio Institucional de la Universitat Politècnica de València Riunet20202020-07-02journal articlehttp://purl.org/coar/resource_type/c_6501VoRhttp://purl.org/coar/version/c_970fb48d4fbd8a85info:eu-repo/semantics/articleapplication/pdfapplication/pdfhttps://riunet.upv.es/handle/10251/178176reponame:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valénciainstname:Universitat Politècnica de València (UPV)InglésengAgencia Estatal de Investigación http://dx.doi.org/10.13039/501100011033 Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016 MAT2017-86659-R DISEÑO DE NANOESTRUCTURAS PLASMONICAS COLOIDALES COMO AGENTES DE CONTRASTE MULTIMODALES PARA BIOIMAGEN Y DIAGNOSTICOMinisterio de Ciencia, Innovación y Universidades https://doi.org/10.13039/100014440 PGC2018-096444-B-I00Agencia Estatal de Investigación http://dx.doi.org/10.13039/501100011033 Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020 RTI2018-095844-B-I00 NUEVOS VECTORES DE ACIDOS NUCLEICOS BASADOS EN MATRICES LIPIDICAS Y NANOPARTICULAS PLASMONICAS DE ORO PARA TERAPIA GENICA CONTRA EL CANCEREUROfusion Consortium EUROfusion Consortium ENR-IFE19.CCFE-01Caja de Ahorros del Mediterráneo https://doi.org/10.13039/100012818 P2018%2FNMT-4389Caja de Ahorros del Mediterráneo https://doi.org/10.13039/100012818 P2018%2FEMT-4437Fondo Nacional de Desarrollo Científico y Tecnológico, Chile https://doi.org/10.13039/501100002850 3190123Fondo Nacional de Desarrollo Científico y Tecnológico, Chile https://doi.org/10.13039/501100002850 11180557Comisión Nacional de Investigación Científica y Tecnológica, Chile https://doi.org/10.13039/501100009068 FB-0807Russian Science Foundation https://doi.org/10.13039/501100006769 19-19-00683open accesshttp://purl.org/coar/access_right/c_abf2Reserva de todos los derechoshttp://rightsstatements.org/vocab/InC/1.0/info:eu-repo/semantics/openAccessoai:riunet.upv.es:10251/1781762026-06-13T07:49:27Z |
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15,300719 |