Sensors based on carbon nanotube field-effect transistors and molecular recognition approaches

The general objective of this thesis is to develop chemical sensors whose sensing capacities are based on the principle of molecular recognition and where the transduction is carried out by single-walled carbon nanotubes (SWCNT).The sensing device used is the carbon nanotube field-effect transistor...

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Detalles Bibliográficos
Autor: Cid Salavert, Cristina Carlota
Tipo de recurso: tesis doctoral
Estado:Versión publicada
Fecha de publicación:2009
País:España
Institución:Universitat Rovira i virgili (URV)
Repositorio:Repositori Institucional de la Universitat Rovira i Virgili
OAI Identifier:oai:urv.cat:TDX:810
Acceso en línea:https://hdl.handle.net/20.500.11797/TDX810
http://hdl.handle.net/10803/9032
Access Level:acceso abierto
Palabra clave:543 - Química analítica
54 - Química
Descripción
Sumario:The general objective of this thesis is to develop chemical sensors whose sensing capacities are based on the principle of molecular recognition and where the transduction is carried out by single-walled carbon nanotubes (SWCNT).The sensing device used is the carbon nanotube field-effect transistor (CNTFET). The new structure of the CNTFET allows nanotubes to be integrated at the surface of the devices, thus exploiting SWCNTs' sensitivity to changes in their environment. The functionalization of SWCNTs with several types of molecular receptors such as antibodies, ion selective membranes, and synthetic receptors, achieve a high selectivity towards the analyte of interest. This thesis shows that CNTFETs can be used for the successful selective detection of different types of target analytes. These can be biomolecules such as antigens, small compounds such as cations or gas-phase compounds such as SO2.