Diversity-Orientated Stereoselective Synthesis through Pd- Catalyzed Switchable Decarboxylative C‒N/C‒S Bond Formation in Allylic Surrogates

Switchable catalytic transformation of reactants can be a powerful approach towards diversity-orientated synthesis from easily available molecular synthons. Herein, an endogenous ligand- controlled, Pd-catalyzed allylic substitution allowing for either selective C‒N or C‒S bond formation using vinyl...

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Detalles Bibliográficos
Autores: Deng, Lei, Kleij, Arjan W., Yang, Weibo
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2018
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2072/356172
Acceso en línea:http://hdl.handle.net/2072/356172
https://doi.org/10.1002/chem.201805295
Access Level:acceso abierto
Palabra clave:54
Descripción
Sumario:Switchable catalytic transformation of reactants can be a powerful approach towards diversity-orientated synthesis from easily available molecular synthons. Herein, an endogenous ligand- controlled, Pd-catalyzed allylic substitution allowing for either selective C‒N or C‒S bond formation using vinylethylene carbonates and N-sulfonylhydrazones as coupling partners has been developed. This versatile methodology provides a facile, diversicating route for the highly chemo- and stereoselective synthesis of functional allylic sulfones or sulfonohydrazides. The newly developed protocol features wide substrate scope (nearly 80 examples), broad functional group tolerance and potential for the late-stage functionalization of bioactive compounds. The isolation and crystallographic analysis of a catalytically competent -allyl Pd complex suggests that the pathway leading to the allylic products proceeds through a different manifold as previously proposed for the functionalization of VECs with nucleophiles.