Field-Free Spin-Orbit Torque Switching in Janus Chromium Dichalcogenides

We predict a very large spin-orbit torque (SOT) capability of magnetic chromium-based transition-metal dichalcogenide (TMD) monolayers in their Janus forms CrXTe, with X = S, Se. The structural inversion symmetry breaking, inherent to Janus structures is responsible for a large SOT response generate...

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Detalles Bibliográficos
Autores: Vojáček, Libor, Medina Dueñas, Joaquin|||0000-0002-9292-8505, Li, Jing|||0000-0002-9283-3821, Ibrahim, Fatima, Manchon, Aurélien, Roche, Stephan|||0000-0003-0323-4665, Chshiev, Mairbek|||0000-0001-9232-7622, Garcia, José H.|||0000-0002-5752-4759
Tipo de recurso: artículo
Fecha de publicación:2024
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:302521
Acceso en línea:https://ddd.uab.cat/record/302521
https://dx.doi.org/urn:doi:10.1021/acs.nanolett.4c03029
Access Level:acceso abierto
Palabra clave:Spin-orbit torque
Transition metal dichalcogenide
2D materials
Van der Waals ferromagnet
Descripción
Sumario:We predict a very large spin-orbit torque (SOT) capability of magnetic chromium-based transition-metal dichalcogenide (TMD) monolayers in their Janus forms CrXTe, with X = S, Se. The structural inversion symmetry breaking, inherent to Janus structures is responsible for a large SOT response generated by giant Rashba splitting, equivalent to that obtained by applying a transverse electric field of ∼100 V nm in non-Janus CrTe, completely out of experimental reach. By performing transport simulations on carefully derived Wannier tight-binding models, Janus systems are found to exhibit an SOT performance comparable to the most efficient two-dimensional materials, while additionally allowing for field-free perpendicular magnetization switching, due to their reduced in-plane symmetry. Altogether, our findings evidence that magnetic Janus TMDs stand as suitable candidates for ultimate SOT-MRAM devices in an ultracompact self-induced SOT scheme.