Polystyrene modified hybrid materials based on ordered mesoporous silica

Organically-modified mesoporous silica materials have been prepared by direct co-condensation of styrylethyltrimethoxysilane (STETMOS) and tetraethylorthosilicate (TEOS) in one-pot synthesis. The polimerizable nature of the styryl-containing precursor induces the formation of anchored polystyrene bl...

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Detalles Bibliográficos
Autores: van Grieken, R., Morales, G., Martin, A., Martinez, F.
Tipo de recurso: artículo
Fecha de publicación:2008
País:España
Institución:Universidad Rey Juan Carlos
Repositorio:BURJC-Digital. Repositorio Institucional de la Universidad Rey Juan Carlos
OAI Identifier:oai:burjcdigital.urjc.es:10115/4008
Acceso en línea:http://hdl.handle.net/10115/4008
Access Level:acceso abierto
Palabra clave:Química
23 Química
Descripción
Sumario:Organically-modified mesoporous silica materials have been prepared by direct co-condensation of styrylethyltrimethoxysilane (STETMOS) and tetraethylorthosilicate (TEOS) in one-pot synthesis. The polimerizable nature of the styryl-containing precursor induces the formation of anchored polystyrene blocks over the silica surface, which are amenable to be functionalized with acid groups via sulfonation. The resultant organosulfonic-modified mesostructured silica materials have exhibited hexagonal long-range mesoscopic arrangement with extended surface areas and narrow mean pore size distributions. The acid capacity of these materials was assessed on the acid-catalyzed reaction test of anisole acylation with acetic anhydride.