High-Throughput Proteomics Sample Preparation Using a 96-Channel Pipettor and Magnetic Pin Device

15 páginas, 8 figuras, 2 tablas

Detalles Bibliográficos
Autores: Roumelioti, Georgia, Montoya, Alex, Fisher, Gemma L. M., Pascual Navarro, Eneko, Woods, Angela, Bennett, Jane, Navaratnam, Naveenan, Gonzalez-Carvajal, Oliver, Birch, Jodie, Pyman, Elizabeth, Yu, Sijia, Gruevska, Aleksandra, Vuillemenot, Luc-Alban, Lushchak, Oleh, Hall, Zoe, Barr, Alexis R., Speck, Christian, Vernia, Santiago, Scott, William R., Gil, Jesus, Aragon, Luis, Fets, Louise, Carling, David, Shliaha, Pavel V.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2026
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/422988
Acceso en línea:http://hdl.handle.net/10261/422988
Access Level:acceso abierto
Palabra clave:PAC
SP3
High-throughput sample preparation
Oasis HLB
Phosphoproteomics
Proteomics
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spelling High-Throughput Proteomics Sample Preparation Using a 96-Channel Pipettor and Magnetic Pin DeviceRoumelioti, GeorgiaMontoya, AlexFisher, Gemma L. M.Pascual Navarro, EnekoWoods, AngelaBennett, JaneNavaratnam, NaveenanGonzalez-Carvajal, OliverBirch, JodiePyman, ElizabethYu, SijiaGruevska, AleksandraVuillemenot, Luc-AlbanLushchak, OlehHall, ZoeBarr, Alexis R.Speck, ChristianVernia, SantiagoScott, William R.Gil, JesusAragon, LuisFets, LouiseCarling, DavidShliaha, Pavel V.PACSP3High-throughput sample preparationOasis HLBPhosphoproteomicsProteomics15 páginas, 8 figuras, 2 tablasHigh-throughput proteomics requires efficient and highly reproducible sample processing, yet workflows─particularly for PTM profiling─remain complex and costly to fully automate. Here, we present a practical intermediate solution using manually operated 96-channel devices: the Gilson Platemaster P220 pipettor and VP Scientific 96-well magnetic pin device. Using this setup, we achieved robust and reproducible phosphoproteomics in a 96-well format, completing protein aggregation capture (PAC/SP3) digestion, desalting, phosphopeptide enrichment, and a second desalting step within 2 days while minimizing operator workload and variability. Several innovations enable this workflow. First, we describe a cost-efficient method to generate 96-well solid-phase extraction plates by directly packing the Oasis HLB sorbent into tapered filter plates. We extensively characterize these plates in terms of loading capacity, lipid removal efficiency, and suitability for high-pH fractionation. Second, we demonstrate that efficient PAC digestion does not require continuous bead suspension; instead, digestion can be achieved by briefly aspirating beads in protease solution, eliminating the need for orbital shaking and simplifying automation. The presented workflow familiarizes users with 96-channel devices and hence serves as a good step toward full automation.Work at the proteomics core facility is supported by MRC LMS core funding (MC-A651-53297).Peer reviewedAmerican Chemical SocietyMRC Laboratory of Medical SciencesVernia, Santiago [0000-0001-6728-5555]Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]202620262026info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501Publisher's versioninfo:eu-repo/semantics/publishedVersionhttp://hdl.handle.net/10261/422988reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Ingléshttps://doi.org/10.1021/acs.jproteome.5c01020Síinfo:eu-repo/semantics/openAccessoai:digital.csic.es:10261/4229882026-05-22T06:33:51Z
dc.title.none.fl_str_mv High-Throughput Proteomics Sample Preparation Using a 96-Channel Pipettor and Magnetic Pin Device
title High-Throughput Proteomics Sample Preparation Using a 96-Channel Pipettor and Magnetic Pin Device
spellingShingle High-Throughput Proteomics Sample Preparation Using a 96-Channel Pipettor and Magnetic Pin Device
Roumelioti, Georgia
PAC
SP3
High-throughput sample preparation
Oasis HLB
Phosphoproteomics
Proteomics
title_short High-Throughput Proteomics Sample Preparation Using a 96-Channel Pipettor and Magnetic Pin Device
title_full High-Throughput Proteomics Sample Preparation Using a 96-Channel Pipettor and Magnetic Pin Device
title_fullStr High-Throughput Proteomics Sample Preparation Using a 96-Channel Pipettor and Magnetic Pin Device
title_full_unstemmed High-Throughput Proteomics Sample Preparation Using a 96-Channel Pipettor and Magnetic Pin Device
title_sort High-Throughput Proteomics Sample Preparation Using a 96-Channel Pipettor and Magnetic Pin Device
dc.creator.none.fl_str_mv Roumelioti, Georgia
Montoya, Alex
Fisher, Gemma L. M.
Pascual Navarro, Eneko
Woods, Angela
Bennett, Jane
Navaratnam, Naveenan
Gonzalez-Carvajal, Oliver
Birch, Jodie
Pyman, Elizabeth
Yu, Sijia
Gruevska, Aleksandra
Vuillemenot, Luc-Alban
Lushchak, Oleh
Hall, Zoe
Barr, Alexis R.
Speck, Christian
Vernia, Santiago
Scott, William R.
Gil, Jesus
Aragon, Luis
Fets, Louise
Carling, David
Shliaha, Pavel V.
author Roumelioti, Georgia
author_facet Roumelioti, Georgia
Montoya, Alex
Fisher, Gemma L. M.
Pascual Navarro, Eneko
Woods, Angela
Bennett, Jane
Navaratnam, Naveenan
Gonzalez-Carvajal, Oliver
Birch, Jodie
Pyman, Elizabeth
Yu, Sijia
Gruevska, Aleksandra
Vuillemenot, Luc-Alban
Lushchak, Oleh
Hall, Zoe
Barr, Alexis R.
Speck, Christian
Vernia, Santiago
Scott, William R.
Gil, Jesus
Aragon, Luis
Fets, Louise
Carling, David
Shliaha, Pavel V.
author_role author
author2 Montoya, Alex
Fisher, Gemma L. M.
Pascual Navarro, Eneko
Woods, Angela
Bennett, Jane
Navaratnam, Naveenan
Gonzalez-Carvajal, Oliver
Birch, Jodie
Pyman, Elizabeth
Yu, Sijia
Gruevska, Aleksandra
Vuillemenot, Luc-Alban
Lushchak, Oleh
Hall, Zoe
Barr, Alexis R.
Speck, Christian
Vernia, Santiago
Scott, William R.
Gil, Jesus
Aragon, Luis
Fets, Louise
Carling, David
Shliaha, Pavel V.
author2_role author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
dc.contributor.none.fl_str_mv MRC Laboratory of Medical Sciences
Vernia, Santiago [0000-0001-6728-5555]
Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]
dc.subject.none.fl_str_mv PAC
SP3
High-throughput sample preparation
Oasis HLB
Phosphoproteomics
Proteomics
topic PAC
SP3
High-throughput sample preparation
Oasis HLB
Phosphoproteomics
Proteomics
description 15 páginas, 8 figuras, 2 tablas
publishDate 2026
dc.date.none.fl_str_mv 2026
2026
2026
dc.type.none.fl_str_mv info:eu-repo/semantics/article
http://purl.org/coar/resource_type/c_6501
Publisher's version
info:eu-repo/semantics/publishedVersion
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/10261/422988
url http://hdl.handle.net/10261/422988
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv https://doi.org/10.1021/acs.jproteome.5c01020

dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.publisher.none.fl_str_mv American Chemical Society
publisher.none.fl_str_mv American Chemical Society
dc.source.none.fl_str_mv reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC
instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str DIGITAL.CSIC. Repositorio Institucional del CSIC
collection DIGITAL.CSIC. Repositorio Institucional del CSIC
repository.name.fl_str_mv
repository.mail.fl_str_mv
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score 15,812455