Subcritical water extraction of phenolic compounds from onion skin wastes (Allium cepa cv. horcal): effect of temperature and solvent properties

The valorization of onion skin wastes (OSW) through the extraction, identification, and quantification of phenolic compounds was studied in this work, using subcritical water in a semicontinuous extractor (2.5 mL/min; 105–180 C; 5 MPa). The extraction of flavonoids resulted to be fast (<30 min) a...

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Detalles Bibliográficos
Autores: Benito Román, Oscar, Blanco Alcalde, Beatriz, Sanz Díez, Mª Teresa, Beltrán Calvo, Sagrario
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2020
País:España
Institución:Universidad de Burgos (UBU)
Repositorio:Repositorio Institucional de la Universidad de Burgos (RIUBU)
OAI Identifier:oai:riubu.ubu.es:10259/6088
Acceso en línea:http://hdl.handle.net/10259/6088
Access Level:acceso abierto
Palabra clave:Onion
Extraction
Subcritical water
Quercetin
Polarity
Valorization
Ingeniería química
Chemical engineering
Descripción
Sumario:The valorization of onion skin wastes (OSW) through the extraction, identification, and quantification of phenolic compounds was studied in this work, using subcritical water in a semicontinuous extractor (2.5 mL/min; 105–180 C; 5 MPa). The extraction of flavonoids resulted to be fast (<30 min) and temperature sensitive (maximum at 145 C; total flavonoids, 27.4 0.9 mg/g dry OSW (DOSW)). The experimental results were fitted to theWeibull model. The influence of the solvent properties on the flavonoids quantification was found to be critical. A precipitate was formed once the extracts cooled down. If removed, a significant fraction of the high temperature extracted flavonoids (as much as 71%, at 180 C) was lost. Such a condition a ected especially those compounds that show extremely low solubility in water at room temperature, whereas quercetin glycosylated derivatives were less a ected by the polarity change of the medium induced by the temperature change. It was demonstrated that it is necessary to re-dissolve the subcritical water extracts by the addition of ethanol, which led to a medium with a polarity equivalent to that obtained with water at high temperature. At 145 C, quercetin (15.4 0.4 mg/g DOSW) and quercetin-40-glucoside (8.4 0.1 mg/g DOSW) accounted for the 90% of the total flavonoids identified. By recovering high added value bioactive compounds from OSW the principles of circular economy were fulfilled, providing a new use for this agricultural waste.