Evidence of zeolitic-like domains in mesostructured aluminosilicates: FTIR spectroscopy of basic probe molecules

The acid properties of mesostructured aluminosilicates synthesized from gel precursors of colloidal ZSM-5 zeolite have been studied by FTIR spectroscopy of basic probe molecules (ammonia, CO and propene). It is shown that these materials possess stronger acid sites with higher thermal stability than...

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Detalles Bibliográficos
Autores: Sánchez Muñoz, María Teresa, Agúndez Rodríguez, Javier, Pérez-Pariente, Joaquín, Márquez Álvarez, Carlos, Onida, B., Garrone, E.
Tipo de recurso: artículo
Fecha de publicación:2007
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/27506
Acceso en línea:http://hdl.handle.net/10261/27506
Access Level:acceso abierto
Palabra clave:mesostructured aluminosilicates
crystalline framework
colloidal ZSM-5
FTIR spectroscopy
Basic probe molecules
Descripción
Sumario:The acid properties of mesostructured aluminosilicates synthesized from gel precursors of colloidal ZSM-5 zeolite have been studied by FTIR spectroscopy of basic probe molecules (ammonia, CO and propene). It is shown that these materials possess stronger acid sites with higher thermal stability than those of conventional A1-MCM-41. These results explain the enhanced m-xylene isomerization activity of these materials and are attributed to the presence of zeolitic-like domains in the aluminosilicate framework.