Optimal model of semi-infinite graphene for ab initio calculations of reactions at graphene edges by the example of zigzag edge reconstruction

We investigate how parameters of the model of semi-infinite graphene based on a graphene nanoribbon under periodic boundary conditions affect the accuracy of ab initio calculations of reactions at graphene edges by the example of the first stage of reconstruction of zigzag graphene edges, formation...

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Detalles Bibliográficos
Autores: Polynskaya, Yulia G.|||0000-0002-9674-0198, Lebedeva, Irina V.|||0000-0002-2880-0275, Knizhnik, Andrey A., Popov, Andrey M.
Tipo de recurso: artículo
Fecha de publicación:2022
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:308914
Acceso en línea:https://ddd.uab.cat/record/308914
https://dx.doi.org/urn:doi:10.1016/j.comptc.2022.113755
Access Level:acceso abierto
Palabra clave:Graphene
Edge reconstruction
Transition state
Structural defect
Density functional theory
Descripción
Sumario:We investigate how parameters of the model of semi-infinite graphene based on a graphene nanoribbon under periodic boundary conditions affect the accuracy of ab initio calculations of reactions at graphene edges by the example of the first stage of reconstruction of zigzag graphene edges, formation of a pentagon-heptagon pair. It is shown that to converge properly the results, the nanoribbon should consist of at least 6 zigzag rows and periodic images of the pair along the nanoribbon axis should be separated by at least 6 hexagons. The converged reaction energy and activation barrier for formation of an isolated pentagon-heptagon pair are found to be -0.15 eV and 1.61 eV, respectively. It is also revealed that such defects reduce the graphene edge magnetization only locally but ordering of spins at opposite nanoribbon edges switches from the antiparallel (antiferromagnetic) to parallel one (ferromagnetic) upon increasing the defect density.