Tuning the thermoelectric response of silicene nanoribbons with vacancies

In this work, we present a thorough study of the thermoelectric properties of silicene nanoribbons in the presence of a random distribution of atomic vacancies. By using a linear approach within the Landauer formalism, we calculate phonon and electron thermal conductances, the electric conductance,...

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Detalles Bibliográficos
Autores: Núñez, C., Saiz Bretín, M., Orellana, P. A., Rosales, L., Domínguez-Adame Acosta, Francisco
Tipo de recurso: artículo
Fecha de publicación:2020
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/6233
Acceso en línea:https://hdl.handle.net/20.500.14352/6233
Access Level:acceso abierto
Palabra clave:538.9
Lattice thermal-conductivity
Landauer formula
Figure
merit
Enhancement
Performance
Transport
Nanowires
Systems
Fano
Thermoelectricity
Silicene Nanoribbons
Thermal transport
Física de materiales
Física del estado sólido
2211 Física del Estado Sólido
Descripción
Sumario:In this work, we present a thorough study of the thermoelectric properties of silicene nanoribbons in the presence of a random distribution of atomic vacancies. By using a linear approach within the Landauer formalism, we calculate phonon and electron thermal conductances, the electric conductance, the Seebeck coefficient and the figure of merit of the nanoribbons. We found a sizable reduction of the phonon thermal conductance as a function of the vacancy concentration over a wide range of temperature. At the same time, the electric properties are not severely deteriorated, leading to an overall remarkable thermoelectric efficiency. We conclude that the incorporation of vacancies paves the way for designing better and more efficient nanoscale thermoelectric devices.