On determining defects identity in carbon nanotubes using charge probes

A metallic carbon nanotube with point-like defects under influence of a local potential due to a point charge probe is theoretically studied. A combination of density functional theory and the Landauer-Büttiker formalism is used to compute the electronic conductance in the zero-voltage limit. From a...

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Detalhes bibliográficos
Autores: Kostyrko, Tomasz, García-Suárez, Víctor M., Wawrzyniak-Adamczewska, M., Ferrer, Jaime
Formato: artículo
Estado:Versión enviada para evaluación y publicación
Fecha de publicación:2016
País:España
Recursos:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/137526
Acesso em linha:http://hdl.handle.net/10261/137526
Access Level:acceso abierto
Palavra-chave:Defects
Scanning probe microscopy
Electronic conductance
Density functional theory
Carbon nanotubes
Descrição
Resumo:A metallic carbon nanotube with point-like defects under influence of a local potential due to a point charge probe is theoretically studied. A combination of density functional theory and the Landauer-Büttiker formalism is used to compute the electronic conductance in the zero-voltage limit. From a collection of the results obtained by varying the probe position around different defects the conductance maps are created. The analysis of the conductance maps allows us to formulate conditions under which several point-like defects (the Stone-Wales defect, a simple carbon vacancy, hydrogen-passivated vacancies) can be distinguished and identified in experiments with the help of scanning probe microscopy.