Ni-Catalysts Supported on N,B-Doped Graphene Aerogels for CO2 Methanation

Methane synthesis from CO2 hydrogenation is a promising approach for CO2 recycling despite challenges such as nickel species loss and sintering. This study investigates reduced graphene aerogels (rGOA) doped with nitrogen (N-rGOA) and boron (B-rGOA) as supports for nickel-based CO2 methanation catal...

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Detalhes bibliográficos
Autores: Sánchez González, María, Villardón Pérez, Alba, Campana Prada, Roberto, Sánchez Silva, María Luz, Dorado Fernández, Fernando, Romero Izquierdo, Amaya
Formato: artículo
Fecha de publicación:2025
País:España
Recursos:Fundación Dialnet. Universidad de La Rioja
Repositorio:RUIdeRA. Repositorio Institucional de la UCLM
OAI Identifier:oai:ruidera.uclm.es:10578/45553
Acesso em linha:https://doi.org/10.1021/acsanm.5c03770
https://hdl.handle.net/10578/45553
Access Level:acceso abierto
Palavra-chave:Aerogels
Graphene-based materials
Heteroatom doping
Methanation
Ni-catalysts
Descrição
Resumo:Methane synthesis from CO2 hydrogenation is a promising approach for CO2 recycling despite challenges such as nickel species loss and sintering. This study investigates reduced graphene aerogels (rGOA) doped with nitrogen (N-rGOA) and boron (B-rGOA) as supports for nickel-based CO2 methanation catalysts. Boron doping (Ni/B-rGOA) improved Ni dispersion and increased the number of active sites through structural and electronic modifications. However, it exhibited slightly lower catalytic performance than nitrogen doping (Ni/N-rGOA), which is attributed to larger Ni particles and higher surface acidity, hindering CO2 activation. ICP and XPS analyses revealed a higher Ni surface segregation in doped samples than in undoped Ni/rGOA. XPS also confirmed the presence of metallic Ni0 and Ni2+ species, with satellite peaks at 861 eV indicative of NiO. Boron doping modified the electronic structure of the carbon support, increasing Ni electron density and catalytic activity. TEM imaging showed well-dispersed Ni nanoparticles (5.9 to 7.3 nm) with no signs of aggregation. Among the tested catalysts, Ni/N-rGOA demonstrated superior CO2 conversion and CH4 selectivity, maintaining stable performance over 60 h of continuous operation. These findings underscore the potential of nitrogen-doped graphene aerogels as robust and efficient supports for the production of CO2 methanation catalysts.