Investigation of Fickian diffusion in the ternary mixture of 1,2,3,4-tetrahydronaphthalene, isobutylbenzene, and dodecane

We present a comprehensive analysis of experimental results obtained for Fickian diffusion in the benchmark ternary liquid mixture of 1,2,3,4-tetrahydronaphthalene, isobutylbenzene, and dodecane (nC(12)) with equal mass fractions. Isothermal diffusion coefficients have been measured by two independe...

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Detalles Bibliográficos
Autores: Mialdun, A., Sechenyh, V., Legros, J. C., Ortiz De Zárate Leira, José María, Shevtsova, V.
Tipo de recurso: artículo
Fecha de publicación:2013
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/33689
Acceso en línea:https://hdl.handle.net/20.500.14352/33689
Access Level:acceso abierto
Palabra clave:536
Taylor dispersion technique
Optical-properties
Light-scattering
Liquid-mixtures
Coefficients
Binary
Interferometry
Cyclohexane
Methanol
Toluene
Termodinámica
2213 Termodinámica
Descripción
Sumario:We present a comprehensive analysis of experimental results obtained for Fickian diffusion in the benchmark ternary liquid mixture of 1,2,3,4-tetrahydronaphthalene, isobutylbenzene, and dodecane (nC(12)) with equal mass fractions. Isothermal diffusion coefficients have been measured by two independent experimental methods: by Taylor dispersion technique, and by a counter flow cell fitted with an optical interferometry device. The experimental diffusion matrices have been critically analyzed regarding the Onsager reciprocal relations, for which we introduce a matrix asymmetry index S-2 that is independent of the frame of reference and the component order.