Poly(carboxylated ether)s as Cement Additives: The Effect of the Addition Method on Hydration Kinetics

Polycarboxylate ether (PCE) superplasticisers have been widely used in cement formulations. However, it is not until recently that several studies have analysed the relationship between the properties and the molecular structure. In the present work, PCEs with different side chain lengths and charge...

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Detalles Bibliográficos
Autores: Beldarrain Pavo, Sara, Goracci, Guido, Sánchez Dolado, Jorge, Barquero Salaberria, Aitor, Leiza Recondo, José Ramón
Tipo de recurso: artículo
Fecha de publicación:2024
País:España
Institución:Universidad del País Vasco
Repositorio:Addi. Archivo Digital para la Docencia y la Investigación
OAI Identifier:oai:addi.ehu.eus:10810/70398
Acceso en línea:http://hdl.handle.net/10810/70398
Access Level:acceso abierto
Palabra clave:hydration kinetics
PCE superplasticizer
direct addition
delayed addition
ordinary portland cement
Descripción
Sumario:Polycarboxylate ether (PCE) superplasticisers have been widely used in cement formulations. However, it is not until recently that several studies have analysed the relationship between the properties and the molecular structure. In the present work, PCEs with different side chain lengths and charge densities synthesised through free radical copolymerisation are used to analyse the effect they have on the hydration of ordinary Portland cement (OPC). It was found that the addition method of these PCEs to the OPC significantly affects the hydration kinetics of the cement paste. When PCEs are added through the direct addition method, a linear dependency between the retardation of hydration and the microstructure of the used PCEs is observed. On the contrary, when PCEs are added through the delayed addition method (PCEs are added to the cement paste 5 min after water), no retardation in hydration is observed, but the rate of hydration is reduced.