Ultralow-dielectric-constant amorphous boron nitride

Decrease in processing speed due to increased resistance and capacitance delay is a major obstacle for the down-scaling of electronics. Minimizing the dimensions of interconnects (metal wires that connect different electronic components on a chip) is crucial for the miniaturization of devices. Inter...

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Autores: Hong, Seokmo, Lee, Chang-Seok|||0000-0002-6078-3874, Lee, Min-Hyun, Lee, Yeongdong|||0000-0001-9749-5270, Ma, Kyung Yeol, Kim, Gwangwoo|||0000-0001-8519-4411, Yoon, Seong In, Ihm, Kyuwook Ihm, Kim, Ki-Jeong, Shin, Tae Joo, Kim, Sang Won, Jeon, Eun-chae|||0000-0002-6951-219X, Jeon, Hansol, Kim, Ju-Young, Lee, Hyung-Ik, Lee, Zonghoon, Antidormi, Aleandro|||0000-0002-5266-8147, Roche, Stephan|||0000-0003-0323-4665, Chhowalla, Manish, Shin, Hyeon-Jin|||0000-0002-6992-6341, Shin, Hyeon Suk|||0000-0003-0495-7443
Tipo de recurso: artículo
Fecha de publicación:2020
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:236030
Acceso en línea:https://ddd.uab.cat/record/236030
https://dx.doi.org/urn:doi:10.1038/s41586-020-2375-9
Access Level:acceso abierto
Palabra clave:Electronic devices
Two-dimensional materials
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spelling Ultralow-dielectric-constant amorphous boron nitrideHong, SeokmoLee, Chang-Seok|||0000-0002-6078-3874Lee, Min-HyunLee, Yeongdong|||0000-0001-9749-5270Ma, Kyung YeolKim, Gwangwoo|||0000-0001-8519-4411Yoon, Seong InIhm, Kyuwook IhmKim, Ki-JeongShin, Tae JooKim, Sang WonJeon, Eun-chae|||0000-0002-6951-219XJeon, HansolKim, Ju-YoungLee, Hyung-IkLee, ZonghoonAntidormi, Aleandro|||0000-0002-5266-8147Roche, Stephan|||0000-0003-0323-4665Chhowalla, ManishShin, Hyeon-Jin|||0000-0002-6992-6341Shin, Hyeon Suk|||0000-0003-0495-7443Electronic devicesTwo-dimensional materialsDecrease in processing speed due to increased resistance and capacitance delay is a major obstacle for the down-scaling of electronics. Minimizing the dimensions of interconnects (metal wires that connect different electronic components on a chip) is crucial for the miniaturization of devices. Interconnects are isolated from each other by non-conducting (dielectric) layers. So far, research has mostly focused on decreasing the resistance of scaled interconnects because integration of dielectrics using low-temperature deposition processes compatible with complementary metal-oxide-semiconductors is technically challenging. Interconnect isolation materials must have low relative dielectric constants (κ values), serve as diffusion barriers against the migration of metal into semiconductors, and be thermally, chemically and mechanically stable. Specifically, the International Roadmap for Devices and Systems recommends the development of dielectrics with κ values of less than 2 by 2028. Existing low-κ materials (such as silicon oxide derivatives, organic compounds and aerogels) have κ values greater than 2 and poor thermo-mechanical properties. Here we report three-nanometre-thick amorphous boron nitride films with ultralow κ values of 1.78 and 1.16 (close to that of air, κ = 1) at operation frequencies of 100 kilohertz and 1 megahertz, respectively. The films are mechanically and electrically robust, with a breakdown strength of 7.3 megavolts per centimetre, which exceeds requirements. Cross-sectional imaging reveals that amorphous boron nitride prevents the diffusion of cobalt atoms into silicon under very harsh conditions, in contrast to reference barriers. Our results demonstrate that amorphous boron nitride has excellent low-κ dielectric characteristics for high-performance electronics. 22020-01-0120202020-01-01Articlehttp://purl.org/coar/resource_type/c_6501AMhttp://purl.org/coar/version/c_ab4af688f83e57aainfo:eu-repo/semantics/articleapplication/pdfhttps://ddd.uab.cat/record/236030https://dx.doi.org/urn:doi:10.1038/s41586-020-2375-9reponame:Dipòsit Digital de Documents de la UABinstname:Universitat Autònoma de BarcelonaInglésengEuropean Commission https://doi.org/10.13039/501100000780 881603European Commission https://doi.org/10.13039/501100000780 785219Agencia Estatal de Investigación https://doi.org/10.13039/501100011033 PCI2018-093120Agencia Estatal de Investigación https://doi.org/10.13039/501100011033 SEV-2017-0706open accesshttp://purl.org/coar/access_right/c_abf2Aquest material està protegit per drets d'autor i/o drets afins. Podeu utilitzar aquest material en funció del que permet la legislació de drets d'autor i drets afins d'aplicació al vostre cas. Per a d'altres usos heu d'obtenir permís del(s) titular(s) de drets.https://rightsstatements.org/vocab/InC/1.0/info:eu-repo/semantics/openAccessoai:ddd.uab.cat:2360302026-06-06T12:50:31Z
dc.title.none.fl_str_mv Ultralow-dielectric-constant amorphous boron nitride
title Ultralow-dielectric-constant amorphous boron nitride
spellingShingle Ultralow-dielectric-constant amorphous boron nitride
Hong, Seokmo
Electronic devices
Two-dimensional materials
title_short Ultralow-dielectric-constant amorphous boron nitride
title_full Ultralow-dielectric-constant amorphous boron nitride
title_fullStr Ultralow-dielectric-constant amorphous boron nitride
title_full_unstemmed Ultralow-dielectric-constant amorphous boron nitride
title_sort Ultralow-dielectric-constant amorphous boron nitride
dc.creator.none.fl_str_mv Hong, Seokmo
Lee, Chang-Seok|||0000-0002-6078-3874
Lee, Min-Hyun
Lee, Yeongdong|||0000-0001-9749-5270
Ma, Kyung Yeol
Kim, Gwangwoo|||0000-0001-8519-4411
Yoon, Seong In
Ihm, Kyuwook Ihm
Kim, Ki-Jeong
Shin, Tae Joo
Kim, Sang Won
Jeon, Eun-chae|||0000-0002-6951-219X
Jeon, Hansol
Kim, Ju-Young
Lee, Hyung-Ik
Lee, Zonghoon
Antidormi, Aleandro|||0000-0002-5266-8147
Roche, Stephan|||0000-0003-0323-4665
Chhowalla, Manish
Shin, Hyeon-Jin|||0000-0002-6992-6341
Shin, Hyeon Suk|||0000-0003-0495-7443
author Hong, Seokmo
author_facet Hong, Seokmo
Lee, Chang-Seok|||0000-0002-6078-3874
Lee, Min-Hyun
Lee, Yeongdong|||0000-0001-9749-5270
Ma, Kyung Yeol
Kim, Gwangwoo|||0000-0001-8519-4411
Yoon, Seong In
Ihm, Kyuwook Ihm
Kim, Ki-Jeong
Shin, Tae Joo
Kim, Sang Won
Jeon, Eun-chae|||0000-0002-6951-219X
Jeon, Hansol
Kim, Ju-Young
Lee, Hyung-Ik
Lee, Zonghoon
Antidormi, Aleandro|||0000-0002-5266-8147
Roche, Stephan|||0000-0003-0323-4665
Chhowalla, Manish
Shin, Hyeon-Jin|||0000-0002-6992-6341
Shin, Hyeon Suk|||0000-0003-0495-7443
author_role author
author2 Lee, Chang-Seok|||0000-0002-6078-3874
Lee, Min-Hyun
Lee, Yeongdong|||0000-0001-9749-5270
Ma, Kyung Yeol
Kim, Gwangwoo|||0000-0001-8519-4411
Yoon, Seong In
Ihm, Kyuwook Ihm
Kim, Ki-Jeong
Shin, Tae Joo
Kim, Sang Won
Jeon, Eun-chae|||0000-0002-6951-219X
Jeon, Hansol
Kim, Ju-Young
Lee, Hyung-Ik
Lee, Zonghoon
Antidormi, Aleandro|||0000-0002-5266-8147
Roche, Stephan|||0000-0003-0323-4665
Chhowalla, Manish
Shin, Hyeon-Jin|||0000-0002-6992-6341
Shin, Hyeon Suk|||0000-0003-0495-7443
author2_role author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv Electronic devices
Two-dimensional materials
topic Electronic devices
Two-dimensional materials
description Decrease in processing speed due to increased resistance and capacitance delay is a major obstacle for the down-scaling of electronics. Minimizing the dimensions of interconnects (metal wires that connect different electronic components on a chip) is crucial for the miniaturization of devices. Interconnects are isolated from each other by non-conducting (dielectric) layers. So far, research has mostly focused on decreasing the resistance of scaled interconnects because integration of dielectrics using low-temperature deposition processes compatible with complementary metal-oxide-semiconductors is technically challenging. Interconnect isolation materials must have low relative dielectric constants (κ values), serve as diffusion barriers against the migration of metal into semiconductors, and be thermally, chemically and mechanically stable. Specifically, the International Roadmap for Devices and Systems recommends the development of dielectrics with κ values of less than 2 by 2028. Existing low-κ materials (such as silicon oxide derivatives, organic compounds and aerogels) have κ values greater than 2 and poor thermo-mechanical properties. Here we report three-nanometre-thick amorphous boron nitride films with ultralow κ values of 1.78 and 1.16 (close to that of air, κ = 1) at operation frequencies of 100 kilohertz and 1 megahertz, respectively. The films are mechanically and electrically robust, with a breakdown strength of 7.3 megavolts per centimetre, which exceeds requirements. Cross-sectional imaging reveals that amorphous boron nitride prevents the diffusion of cobalt atoms into silicon under very harsh conditions, in contrast to reference barriers. Our results demonstrate that amorphous boron nitride has excellent low-κ dielectric characteristics for high-performance electronics.
publishDate 2020
dc.date.none.fl_str_mv 2
2020-01-01
2020
2020-01-01
dc.type.none.fl_str_mv Article
http://purl.org/coar/resource_type/c_6501
AM
http://purl.org/coar/version/c_ab4af688f83e57aa
dc.type.openaire.fl_str_mv info:eu-repo/semantics/article
format article
dc.identifier.none.fl_str_mv https://ddd.uab.cat/record/236030
https://dx.doi.org/urn:doi:10.1038/s41586-020-2375-9
url https://ddd.uab.cat/record/236030
https://dx.doi.org/urn:doi:10.1038/s41586-020-2375-9
dc.language.none.fl_str_mv Inglés
eng
language_invalid_str_mv Inglés
language eng
dc.relation.none.fl_str_mv European Commission https://doi.org/10.13039/501100000780 881603
European Commission https://doi.org/10.13039/501100000780 785219
Agencia Estatal de Investigación https://doi.org/10.13039/501100011033 PCI2018-093120
Agencia Estatal de Investigación https://doi.org/10.13039/501100011033 SEV-2017-0706
dc.rights.none.fl_str_mv open access
http://purl.org/coar/access_right/c_abf2
https://rightsstatements.org/vocab/InC/1.0/
dc.rights.openaire.fl_str_mv info:eu-repo/semantics/openAccess
rights_invalid_str_mv open access
http://purl.org/coar/access_right/c_abf2
https://rightsstatements.org/vocab/InC/1.0/
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
dc.source.none.fl_str_mv reponame:Dipòsit Digital de Documents de la UAB
instname:Universitat Autònoma de Barcelona
instname_str Universitat Autònoma de Barcelona
reponame_str Dipòsit Digital de Documents de la UAB
collection Dipòsit Digital de Documents de la UAB
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