Nonlinear optical rectification and optical bistability in a coupled asymmetric quantum dot-metal nanoparticle hybrid

We study the optical response of a coupled asymmetric semiconductor quantum dot-spherical metal nanoparticle structure. The asymmetric quantum dot has permanent electric dipole moments that also interact with light. We derive the density matrix equations for the system including the modification of...

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Detalles Bibliográficos
Autores: Carreño Sánchez, Fernando, Antón Revilla, Miguel Ángel, Paspalakis, Emmanuel
Tipo de recurso: artículo
Fecha de publicación:2018
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/13030
Acceso en línea:https://hdl.handle.net/20.500.14352/13030
Access Level:acceso abierto
Palabra clave:539.2:620.1
530.145
535.317.2
Optical rectification
Electric dipole moments
Optical bistability
Nanoparticles
Population inversion
Plasmonics
Plasmons
Excitons
Quantum dots
Física del estado sólido
Óptica (Física)
Óptica física, óptica cuántica
2211 Física del Estado Sólido
2209.19 Óptica Física
2209.19 Óptica física
Descripción
Sumario:We study the optical response of a coupled asymmetric semiconductor quantum dot-spherical metal nanoparticle structure. The asymmetric quantum dot has permanent electric dipole moments that also interact with light. We derive the density matrix equations for the system including the modification of the electric field and the exciton-plasmon coupling. We emphasize on the effects of the nonlinear optical rectification and controlled optical bistability and analyze these phenomena for different values of the light intensity and different distances between the quantum dot and the metal nanoparticle. We show that when the system is set in a situation where optical bistability can be produced, the optical rectification of the hybrid system is bivalued. We also analyze the slow-down to reach the steady state when the system is driven close and far from the turning points.