The cytotoxin α‐sarcin behaves as a cyclizing ribonuclease

The hydrolysis of adenylyl(3PC5P)adenosine (ApA) and guanylyl(3PC5P)adenosine (GpA) dinucleotides by the cytotoxic protein K-sarcin has been studied. Quantitative analysis of the reaction has been performed through reversephase chromatographic (HPLC) separation of the resulting products. The hydroly...

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Detalles Bibliográficos
Autores: Lacadena García-Gallo, Francisco Javier, Martínez Del Pozo, Álvaro, Valle Lacadena, Martínez Ruiz, Antonio, Mancheño Gómez, José Miguel, Oñaderra Sánchez, Mercedes, Gavilanes Franco, José Gregorio
Tipo de recurso: artículo
Fecha de publicación:1998
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/103372
Acceso en línea:https://hdl.handle.net/20.500.14352/103372
Access Level:acceso abierto
Palabra clave:577.1
Dinucleotide
Ribonucleolytic activity
Ribosome-inactivating protein
Ribotoxin
Bioquímica (Química)
2302 Bioquímica
Descripción
Sumario:The hydrolysis of adenylyl(3PC5P)adenosine (ApA) and guanylyl(3PC5P)adenosine (GpA) dinucleotides by the cytotoxic protein K-sarcin has been studied. Quantitative analysis of the reaction has been performed through reversephase chromatographic (HPLC) separation of the resulting products. The hydrolysis of the 3P-5P phosphodiester bond of these substrates yields the 2P-3P cyclic mononucleotide; this intermediate is converted into the corresponding 3P-monophosphate derivative as the final product of the reaction. The values of the apparent Michaelis constant (KM), kcat and kcat/ KM have also been calculated. The obtained results fit into a twostep mechanism for the enzymatic activity of K-sarcin and allow to consider this protein as a cyclizing RNase. z 1998 Federation of European Biochemical Societies.