Catalytic VOCs elimination over copper and cerium oxide modified mesoporous SBA-15 silica

[EN] Copper and cerium oxide bi-component materials with different Cu/Ce ratio were prepared using ordered SBA-15 silica as a support and compared with their bulk analogs. The samples were characterized by nitrogen physisorption, XRD, UV-Vis, FTIR, XPS, Raman spectroscopy and TPR with hydrogen. Cycl...

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Detalles Bibliográficos
Autores: Tsoncheva, Tanya, Issa, Gloria, Dimitrov, M., Popova, Margarita, Hernández Morejudo, Selene, Kovacheva, Daniela, Atanasova, Genoveva, Blasco Lanzuela, Teresa|||0000-0002-8115-4241, López Nieto, José Manuel|||0000-0002-6960-3219
Tipo de recurso: artículo
Fecha de publicación:2013
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/100072
Acceso en línea:https://riunet.upv.es/handle/10251/100072
Access Level:acceso abierto
Palabra clave:VOCs oxidation
Copper and cerium oxide catalysts
SBA-15 support
Catalytic sites
Descripción
Sumario:[EN] Copper and cerium oxide bi-component materials with different Cu/Ce ratio were prepared using ordered SBA-15 silica as a support and compared with their bulk analogs. The samples were characterized by nitrogen physisorption, XRD, UV-Vis, FTIR, XPS, Raman spectroscopy and TPR with hydrogen. Cyclohexanol conversion was used as a catalytic test to obtain more information for the surface properties of the supported materials. The catalytic properties of the samples were studied in VOCs oxidation using toluene and ethyl acetate as probe molecules. A strong effect of mesoporous silica support and samples composition on the formation of catalytic sites was established. (C) 2012 Elsevier B.V. All rights reserved.