Transcript profiling of jasmonate-elicited Taxus cells reveals a β-phenylalanine-CoA ligase

Plant cell cultures constitute eco-friendly biotechnological platforms for the production of plant secondary metabolites with pharmacological activities, as well as a suitable system for extending our knowledge of secondary metabolism. Despite the high added value of taxol and the importance of taxa...

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Autores: Ramírez Estrada, Karla, Altabella, Teresa, Onrubia Ibáñez, Miriam, 1982-, Moyano Claramunt, Elisabet, Notredame, Cedric, Osuna, Lidia, Vanden Bossche, Robin, Goossens, Alain, Cusidó Vidal, Rosa M., Palazón Barandela, Javier
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2016
País:España
Institución:Universitat Pompeu Fabra
Repositorio:Repositorio Digital de la UPF
OAI Identifier:oai:repositori.upf.edu:10230/27997
Acceso en línea:http://hdl.handle.net/10230/27997
http://dx.doi.org/10.1111/pbi.12359
Access Level:acceso abierto
Palabra clave:CDNA-AFLP
CoA ligase
Methyl jasmonate
Beta-phenylalanine
Taxol
Taxus baccata
Cell cultures
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spelling Transcript profiling of jasmonate-elicited Taxus cells reveals a β-phenylalanine-CoA ligaseRamírez Estrada, Karla Altabella, TeresaOnrubia Ibáñez, Miriam, 1982-Moyano Claramunt, ElisabetNotredame, CedricOsuna, LidiaVanden Bossche, RobinGoossens, AlainCusidó Vidal, Rosa M.Palazón Barandela, JavierCDNA-AFLPCoA ligaseMethyl jasmonateBeta-phenylalanineTaxolTaxus baccataCell culturesPlant cell cultures constitute eco-friendly biotechnological platforms for the production of plant secondary metabolites with pharmacological activities, as well as a suitable system for extending our knowledge of secondary metabolism. Despite the high added value of taxol and the importance of taxanes as anticancer compounds, several aspects of their biosynthesis remain unknown. In this work, a genomewide expression analysis of jasmonate-elicited Taxus baccata cell cultures by complementary DNA-amplified fragment length polymorphism (cDNA-AFLP) indicated a correlation between an extensive elicitor-induced genetic reprogramming and increased taxane production in the targeted cultures. Subsequent in silico analysis allowed us to identify 15 genes with a jasmonate-induced differential expression as putative candidates for genes encoding enzymes involved in five unknown steps of taxane biosynthesis. Among them, the TB768 gene showed a strong homology, including a very similar predicted 3D structure, with other genes previously reported to encode acyl-CoA ligases, thus suggesting a role in the formation of the taxol lateral chain. Functional analysis confirmed that the TB768 gene encodes an acyl-CoA ligase that localizes to the cytoplasm and is able to convert β-phenylalanine, as well as coumaric acid, into their respective derivative CoA esters. β-phenylalanyl-CoA is attached to baccatin III in one of the last steps of the taxol biosynthetic pathway. The identification of this gene will contribute to the establishment of sustainable taxol production systems through metabolic engineering or synthetic biology approaches.This research has been supported by two grants from the Spanish MINECO (BIO2011-29856-C02-01 and AGL2013-43522-R) and a grant from Generalitat de Catalunya (2014SGR1434).Wiley201720172016info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionapplication/pdfapplication/pdfhttp://hdl.handle.net/10230/27997http://dx.doi.org/10.1111/pbi.12359reponame:Repositorio Digital de la UPFinstname:Universitat Pompeu FabraInglésPlant Biotechnology Journal. 2016;14(1):85-96info:eu-repo/grantAgreement/ES/3PN/BIO2011-29856-C02-01info:eu-repo/grantAgreement/ES/1PE/AGL2013-43522-R© Society for Experimental Biology, Association of Applied Biologists and John Wiley & Sons Ltd. All articles accepted from 1st January 2016 (date of flip) are published under the terms of the Creative Commons Attribution License. Articles accepted before this date were published under the agreement as stated in the final article.https://creativecommons.org/licenses/by/3.0/info:eu-repo/semantics/openAccessoai:repositori.upf.edu:10230/279972026-06-12T07:21:37Z
dc.title.none.fl_str_mv Transcript profiling of jasmonate-elicited Taxus cells reveals a β-phenylalanine-CoA ligase
title Transcript profiling of jasmonate-elicited Taxus cells reveals a β-phenylalanine-CoA ligase
spellingShingle Transcript profiling of jasmonate-elicited Taxus cells reveals a β-phenylalanine-CoA ligase
Ramírez Estrada, Karla
CDNA-AFLP
CoA ligase
Methyl jasmonate
Beta-phenylalanine
Taxol
Taxus baccata
Cell cultures
title_short Transcript profiling of jasmonate-elicited Taxus cells reveals a β-phenylalanine-CoA ligase
title_full Transcript profiling of jasmonate-elicited Taxus cells reveals a β-phenylalanine-CoA ligase
title_fullStr Transcript profiling of jasmonate-elicited Taxus cells reveals a β-phenylalanine-CoA ligase
title_full_unstemmed Transcript profiling of jasmonate-elicited Taxus cells reveals a β-phenylalanine-CoA ligase
title_sort Transcript profiling of jasmonate-elicited Taxus cells reveals a β-phenylalanine-CoA ligase
dc.creator.none.fl_str_mv Ramírez Estrada, Karla
Altabella, Teresa
Onrubia Ibáñez, Miriam, 1982-
Moyano Claramunt, Elisabet
Notredame, Cedric
Osuna, Lidia
Vanden Bossche, Robin
Goossens, Alain
Cusidó Vidal, Rosa M.
Palazón Barandela, Javier
author Ramírez Estrada, Karla
author_facet Ramírez Estrada, Karla
Altabella, Teresa
Onrubia Ibáñez, Miriam, 1982-
Moyano Claramunt, Elisabet
Notredame, Cedric
Osuna, Lidia
Vanden Bossche, Robin
Goossens, Alain
Cusidó Vidal, Rosa M.
Palazón Barandela, Javier
author_role author
author2 Altabella, Teresa
Onrubia Ibáñez, Miriam, 1982-
Moyano Claramunt, Elisabet
Notredame, Cedric
Osuna, Lidia
Vanden Bossche, Robin
Goossens, Alain
Cusidó Vidal, Rosa M.
Palazón Barandela, Javier
author2_role author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv CDNA-AFLP
CoA ligase
Methyl jasmonate
Beta-phenylalanine
Taxol
Taxus baccata
Cell cultures
topic CDNA-AFLP
CoA ligase
Methyl jasmonate
Beta-phenylalanine
Taxol
Taxus baccata
Cell cultures
description Plant cell cultures constitute eco-friendly biotechnological platforms for the production of plant secondary metabolites with pharmacological activities, as well as a suitable system for extending our knowledge of secondary metabolism. Despite the high added value of taxol and the importance of taxanes as anticancer compounds, several aspects of their biosynthesis remain unknown. In this work, a genomewide expression analysis of jasmonate-elicited Taxus baccata cell cultures by complementary DNA-amplified fragment length polymorphism (cDNA-AFLP) indicated a correlation between an extensive elicitor-induced genetic reprogramming and increased taxane production in the targeted cultures. Subsequent in silico analysis allowed us to identify 15 genes with a jasmonate-induced differential expression as putative candidates for genes encoding enzymes involved in five unknown steps of taxane biosynthesis. Among them, the TB768 gene showed a strong homology, including a very similar predicted 3D structure, with other genes previously reported to encode acyl-CoA ligases, thus suggesting a role in the formation of the taxol lateral chain. Functional analysis confirmed that the TB768 gene encodes an acyl-CoA ligase that localizes to the cytoplasm and is able to convert β-phenylalanine, as well as coumaric acid, into their respective derivative CoA esters. β-phenylalanyl-CoA is attached to baccatin III in one of the last steps of the taxol biosynthetic pathway. The identification of this gene will contribute to the establishment of sustainable taxol production systems through metabolic engineering or synthetic biology approaches.
publishDate 2016
dc.date.none.fl_str_mv 2016
2017
2017
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/10230/27997
http://dx.doi.org/10.1111/pbi.12359
url http://hdl.handle.net/10230/27997
http://dx.doi.org/10.1111/pbi.12359
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv Plant Biotechnology Journal. 2016;14(1):85-96
info:eu-repo/grantAgreement/ES/3PN/BIO2011-29856-C02-01
info:eu-repo/grantAgreement/ES/1PE/AGL2013-43522-R
dc.rights.none.fl_str_mv https://creativecommons.org/licenses/by/3.0/
info:eu-repo/semantics/openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by/3.0/
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Wiley
publisher.none.fl_str_mv Wiley
dc.source.none.fl_str_mv reponame:Repositorio Digital de la UPF
instname:Universitat Pompeu Fabra
instname_str Universitat Pompeu Fabra
reponame_str Repositorio Digital de la UPF
collection Repositorio Digital de la UPF
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repository.mail.fl_str_mv
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