Cyclopropane-Alkene Metathesis by Gold(I)-Catalyzed Decarbenation of Persistent Cyclopropanes

A gold(I)-catalyzed cyclopropane-alkene metathesis has been demonstrated with two new families of cyclopropane derivatives of naphthalene and phenanthrene (benzo-fused norcaradienes). In this process, metal carbene units are transferred from a persistent cyclopropane to an alkene, upon release of na...

ver descrição completa

Detalhes bibliográficos
Autores: Mato, Mauro, Martín-Torres, Inmaculada, Herlé, Bart, Echavarren, Antonio M.
Tipo de documento: artigo
Estado:Versión aceptada para publicación
Data de publicação:2019
País:España
Recursos:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositório:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2072/355600
Acesso em linha:http://hdl.handle.net/2072/355600
https://doi.org/10.1039/C9OB00359B
Access Level:Acceso aberto
Palavra-chave:54
Descrição
Resumo:A gold(I)-catalyzed cyclopropane-alkene metathesis has been demonstrated with two new families of cyclopropane derivatives of naphthalene and phenanthrene (benzo-fused norcaradienes). In this process, metal carbene units are transferred from a persistent cyclopropane to an alkene, upon release of naphthalene or phenanthrene, allowing the diastereoselective synthesis of a wide range of aryl and vinyl cyclopropanes.