Ballistic Phonons in Ultrathin Nanowires

According to Fourier's law, a temperature difference across a material results in a linear temperature profile and a thermal conductance that decreases inversely proportional to the system length. These are the hallmarks of diffusive heat flow. Here, we report heat flow in ultrathin (25 nm) GaP...

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Detalles Bibliográficos
Autores: Vakulov, Daniel, Gireesan, Subash, Swinkels, Milo Y., Chavez, Ruben, Vogelaar, Tom, Torres Alvarez, Pol|||0000-0003-2544-5850, Campo, Alessio, De Luca, Marta|||0000-0001-6061-3261, Verheijen, Marcel A., Koelling, Sebastian, Gagliano, Luca, Haverkort, Jos E. M., Alvarez, F. Xavier|||0000-0001-6746-2144, Bobbert, Peter A., Zardo, Ilaria|||0000-0002-8685-2305, Bakkers, Erik P. A. M.
Tipo de recurso: artículo
Fecha de publicación:2020
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:226283
Acceso en línea:https://ddd.uab.cat/record/226283
https://dx.doi.org/urn:doi:10.1021/acs.nanolett.0c00320
Access Level:acceso abierto
Palabra clave:Nanowires
GaP
Heat transport
Ballistic phonons
Raman spectroscopy
Descripción
Sumario:According to Fourier's law, a temperature difference across a material results in a linear temperature profile and a thermal conductance that decreases inversely proportional to the system length. These are the hallmarks of diffusive heat flow. Here, we report heat flow in ultrathin (25 nm) GaP nanowires in the absence of a temperature gradient within the wire and find that the heat conductance is independent of wire length. These observations deviate from Fourier's law and are direct proof of ballistic heat flow, persisting for wire lengths up to at least 15 μm at room temperature. When doubling the wire diameter, a remarkably sudden transition to diffusive heat flow is observed. The ballistic heat flow in the ultrathin wires can be modeled within Landauer's formalism by ballistic phonons with an extraordinarily long mean free path.