Dynamic Raman Spectroelectrochemistry of Single Walled Carbon Nanotubes modified electrodes using a Langmuir-Schaefer method

Raman spectroelectrochemistry is a fundamental technique to characterize single walled carbon nanotube (SWCNT) films. In this work, we have performed the study of SWCNT films transferred to a glassy carbon electrode using a Langmuir-Schaefer method. Langmuir balance has allowed us to control the cha...

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Detalles Bibliográficos
Autores: Ibáñez Martínez, David, Romero, Edna Cecilia, Colina, Álvaro, Heras, Aránzazu
Tipo de recurso: artículo
Estado:Versión enviada para evaluación y publicación
Fecha de publicación:2014
País:España
Institución:Universidad de Burgos (UBU)
Repositorio:Repositorio Institucional de la Universidad de Burgos (RIUBU)
OAI Identifier:oai:riubu.ubu.es:10259/3853
Acceso en línea:http://hdl.handle.net/10259/3853
Access Level:acceso abierto
Palabra clave:Spectroelectrochemistry
Electrochemistry
Raman spectroscopy
Langmuir balance
Single walled carbon nanotube
Química analítica
Chemistry, Analytic
Descripción
Sumario:Raman spectroelectrochemistry is a fundamental technique to characterize single walled carbon nanotube (SWCNT) films. In this work, we have performed the study of SWCNT films transferred to a glassy carbon electrode using a Langmuir-Schaefer method. Langmuir balance has allowed us to control the characteristics of the film that can be easily transferred to the electrode support. Time-resolved Raman spectroelectrochemistry experiments at scan rates between 20 and 400 mV s−1 were done in two different solvents, water and acetonitrile. Spectroscopic results indicate that electron transfer of carbon nanotubes is a very fast process. The electrochemical process is reversible in acetonitrile and, on the contrary, nanotubes are degraded when the characterization is performed in water being the degradation independent on the scan rate.