Electrochemically assisted adsorption/desorption of bentazone on activated carbon cloth

This paper investigates the use of electrochemical techniques for the removal of a common herbicide, bentazone, from water streams using a carbon-based electrode. Activated carbon cloth with high surface area and narrow micropores was used as electrode. For a better understanding of the process, ads...

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Detalhes bibliográficos
Autores: Ovín Ania, María Concepción, Béguin, François
Formato: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2007
País:España
Recursos:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/98676
Acesso em linha:http://hdl.handle.net/10261/98676
Access Level:acceso abierto
Palavra-chave:Electrosorption
Electrodesorption
Activated carbon cloth
Pesticides
Liquid phase adsorption
Descrição
Resumo:This paper investigates the use of electrochemical techniques for the removal of a common herbicide, bentazone, from water streams using a carbon-based electrode. Activated carbon cloth with high surface area and narrow micropores was used as electrode. For a better understanding of the process, adsorption was investigated under both open circuit and controlled polarization conditions, the latter in anodic and cathodic directions. It was found that anodic polarization enhances the kinetics of adsorption of the herbicide on the carbon cloth, the extent of which is strongly related to the applied current value. At converse, cathodic polarization induces the reversible desorption of the compound. Moreover, in-situ UV spectra recording on the solution did not show any structural change of the herbicide upon polarization, demonstrating the reversibility of the process for the regeneration of the adsorbent and the recovery of the compound. Based on these experiments, a mechanism is proposed to interpret the reversible sorption of bentazone under polarization.