Novel developments in the Diffusive Gradient in Thin films (DGT) technique for the determination of bioavailable mercury and other trace metals in aquatic and terrestrial environments

This thesis is focused on the use of the Diffusive Gradient in thin film (DGT) technique for the analysis of bioavailable mercury and other trace metals in water and soil. Homemade DGT devices using a selective ion-exchange resin, and a polyacrylamide gel as the diffusive layer using an open resin (...

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Detalles Bibliográficos
Autor: Turull López, Marta
Tipo de recurso: tesis doctoral
Estado:Versión publicada
Fecha de publicación:2019
País:España
Institución:CBUC, CESCA
Repositorio:TDR. Tesis Doctorales en Red
OAI Identifier:oai:www.tdx.cat:10803/668780
Acceso en línea:http://hdl.handle.net/10803/668780
Access Level:acceso abierto
Palabra clave:DGT technique
Diffusive Gradient in Thin film
Gradient de difusió en capa fina
Gradiente de difusión en capa fina
Mercury
Mercuri
Mercurio
Trace metals
Traces de metalls
Trazas de metales
Water
Aigua
Agua
Soil
Sòl
Suelo
Bioavailability
Biodisponibilitat
Biodisponibilidad
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Descripción
Sumario:This thesis is focused on the use of the Diffusive Gradient in thin film (DGT) technique for the analysis of bioavailable mercury and other trace metals in water and soil. Homemade DGT devices using a selective ion-exchange resin, and a polyacrylamide gel as the diffusive layer using an open resin (>5 nm), have been used to determine the labile Hg in different aquatic systems, concretely in the Ebro river (Spain) and Tully river (Australia). Besides, a new design of DGT using a bis-acrylamide as a restricted layer (<1 nm) has been performed to determine different species of Hg in agricultural soils. On the other hand, using Chelex-100 as the resin in the DGT devices allowed the analysis of bioavailable trace metals and further correlation with the plant uptake, specifically by lettuces (Lactuca sativa)