Treatment of real effluents from the pharmaceutical industry: A comparison between Fenton oxidation and conductive-diamond electro-oxidation

Wastewater produced in pharmaceutical manufacturing plants (PMPs), especially the one coming from organic-synthesis facilities, is characterized by its large variability due to the wide range of solvents and chemical reagents used in the different stages of the production of medicines. Normally, the...

ver descrição completa

Detalhes bibliográficos
Autores: Pérez Serrano, José Fernando, Llanos López, Javier, Sáez Jiménez, Cristina, López Gómez, Conrado, Cañizares Cañizares, Pablo, Rodrigo Rodrigo, Manuel Andrés
Formato: artículo
Fecha de publicación:2017
País:España
Recursos:Universidad de Castilla-La Mancha
Repositorio:RUIdeRA. Repositorio Institucional de la UCLM
OAI Identifier:oai:ruidera.uclm.es:10578/17614
Acesso em linha:http://hdl.handle.net/10578/17614
Access Level:acceso abierto
Palavra-chave:Pharmaceutical manufacturing process
Wastewater
Real industrial effluents
Fenton oxidation
Conductive diamond electro-oxidation
Proceso de fabricación farmacéutica
Aguas residuales
Efluentes industriales reales
Oxidación de Fenton
Electro-oxidación conductora de diamantes
Descrição
Resumo:Wastewater produced in pharmaceutical manufacturing plants (PMPs), especially the one coming from organic-synthesis facilities, is characterized by its large variability due to the wide range of solvents and chemical reagents used in the different stages of the production of medicines. Normally, the toxicity of the organic compounds prevent the utilization of biological processes and more powerful treatments are needed becoming advanced oxidation processes (AOPs) a valid alternative. In this work, the efficiency in abatement of pollution by Fenton oxidation (FO) and conductive-diamond electro- oxidation (CDEO) are compared in the treatment of 60 real effluents coming from different processes carried out in a pharmaceutical facility, using standardized tests. In 80% of the samples, CDEO was found to be more efficient than FO and in the remaining 20%, coagulation was found to exhibit a great significance in the COD abatement mechanism during FO, pointing out the effectiveness of the oxidation promoted by the electrochemical technology. Mean oxidation state of carbon was found to be a relevant parameter to understand the behavior of the oxidation technologies. It varied inversely proportional to efficiency in FO and it showed practically no influence in the case of CDEO.