Non-covalent graphene nanobuds from mono- and tripodal binding motifs

Graphene nanobuds were prepared via the non-covalent anchoring of C60-based molecules endowed with one or three pyrene units. TGA, FTIR, UV-Vis and TEM investigations confirmed the nanohybrids formation. For the two molecular derivatives, striking differences were determined in their interaction wit...

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Detalhes bibliográficos
Autores: Garrido, Marina, Calbo, Joaquín, Rodríguez Pérez, Laura, Aragó, Juan, Ortí, Enrique, Herranz, M.Angeles, Martín, Nazario
Formato: artículo
Fecha de publicación:2017
País:España
Recursos:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/18398
Acesso em linha:https://hdl.handle.net/20.500.14352/18398
Access Level:acceso abierto
Palavra-chave:547
Química orgánica (Química)
2306 Química Orgánica
Descrição
Resumo:Graphene nanobuds were prepared via the non-covalent anchoring of C60-based molecules endowed with one or three pyrene units. TGA, FTIR, UV-Vis and TEM investigations confirmed the nanohybrids formation. For the two molecular derivatives, striking differences were determined in their interaction with graphene or carbon surfaces by Raman, cyclic voltammetry and molecular mechanics calculations, revealing the important role of pyrene adsorption in the electronic properties of the nanohybrids.