Molecular Determinants for Cyclo-oligosaccharide-based Nanoparticle-mediated Effective siRNA Transfection

Aim: To study the structural requirements that a cyclooligosaccharide-based nanoparticle must fulfill to be an efficient siRNA transfection vector. Materials & methods: siRNA protection from degradation by RNAses, transfection efficiency and the thermodynamic parameters of the nanoparticle/siRNA...

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Detalles Bibliográficos
Autores: Manzanares, Darío, Araya Durán, Ingrid, Gallego Yerga, Laura, Játiva, Pablo, Márquez Miranda, Valeria, Canan, Jonathan, Jiménez Blanco, José Luis, Ortiz Mellet, Carmen, González Nilo, Fernando Danilo, García Fernández, José Manuel, Ceña, Valentín
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2017
País:España
Institución:Universidad de Sevilla (US)
Repositorio:idUS. Depósito de Investigación de la Universidad de Sevilla
OAI Identifier:oai:idus.us.es:11441/140690
Acceso en línea:https://hdl.handle.net/11441/140690
https://doi.org/10.2217/nnm-2017-0123
Access Level:acceso abierto
Palabra clave:Endosomal escape
Molecular modeling
Molecular nanoparticle
Protection from RNAses
Protein knock down
siRNA transfection
Descripción
Sumario:Aim: To study the structural requirements that a cyclooligosaccharide-based nanoparticle must fulfill to be an efficient siRNA transfection vector. Materials & methods: siRNA protection from degradation by RNAses, transfection efficiency and the thermodynamic parameters of the nanoparticle/siRNA interactions were studied on pairs of amphiphilic molecules using biochemical techniques and molecular dynamics. Results: The lower the siRNA solvent accessible surface area in the presence of the nanoparticle, higher the protection from RNAse-mediated degradation in the corresponding nanocomplex; a moderate nanoparticle/siRNA binding energy value further facilitates reversible complexation and binding to the target cellular mRNA. Conclusion: The use, in advance, of these parameters will provide a useful indication of the potential of a molecular nanoparticle as siRNA transfecting vector.