Modeling the thermopower of icosahedral Al_(63)Cu_(25)Fe_(12) quasicrystals: spectral fine structure

On the basis of a realistic model for the spectral conductivity, obtained from a proper combination of tunneling spectroscopy [R. Escudero , J. Phys.: Condens. Matter 11, 383 (1999)] and transport measurements, we derive a closed analytical expression for the Seebeck coefficient, satisfactorily desc...

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Detalles Bibliográficos
Autor: Maciá Barber, Enrique Alfonso
Tipo de recurso: artículo
Fecha de publicación:2004
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/52113
Acceso en línea:https://hdl.handle.net/20.500.14352/52113
Access Level:acceso abierto
Palabra clave:538.9
Al-Cu-Fe
Electronic transport-properties
Thermoelectric properties
Conductivity
Alloys
Phases
Law
Approximants
Dependence
Wiedemann
Física de materiales
Física del estado sólido
2211 Física del Estado Sólido
Descripción
Sumario:On the basis of a realistic model for the spectral conductivity, obtained from a proper combination of tunneling spectroscopy [R. Escudero , J. Phys.: Condens. Matter 11, 383 (1999)] and transport measurements, we derive a closed analytical expression for the Seebeck coefficient, satisfactorily describing its temperature dependence over a wide temperature range. The relative importance of thermal broadening effects and the temperature dependence of chemical potential in the thermopower curve is quantitatively discussed. By comparing the obtained analytical results with the experimental S(T) curve evidence for band structure effects in the thermopower is reported.