Elimination of the reaction rate 'scale effect': application of the Lagrangian reactive particle-tracking method to simulate mixing-limited, field-scale biodegradation at the Schoolcraft (MI, USA) site

This is the peer reviewed version of the following article: [Ding, D., Benson, D. A., Fernàndez‐Garcia, D., Henri, C. V., Hyndman, D. W., Phanikumar, M. S., & Bolster, D. (2017). Elimination of the reaction rate “scale effect”: Application of the Lagrangian reactive particle‐tracking method to s...

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Detalles Bibliográficos
Autores: Dong, Ding, Benson, David A., Fernández García, Daniel|||0000-0002-4667-3003, Henri, Christopher Vincent, Hyndman, David W., Phanikumar, Mantha S., Bolster, Diogo
Tipo de recurso: artículo
Fecha de publicación:2017
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/115474
Acceso en línea:https://hdl.handle.net/2117/115474
https://dx.doi.org/10.1002/2017WR021103
Access Level:acceso abierto
Palabra clave:Bioremediation
Particle tracking
Reactive transport
Scale effect
Bioremediació
Àrees temàtiques de la UPC::Enginyeria civil::Geologia::Hidrologia subterrània
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spelling Elimination of the reaction rate 'scale effect': application of the Lagrangian reactive particle-tracking method to simulate mixing-limited, field-scale biodegradation at the Schoolcraft (MI, USA) siteDong, DingBenson, David A.Fernández García, Daniel|||0000-0002-4667-3003Henri, Christopher VincentHyndman, David W.Phanikumar, Mantha S.Bolster, DiogoBioremediationBioremediationParticle trackingReactive transportScale effectBioremediacióÀrees temàtiques de la UPC::Enginyeria civil::Geologia::Hidrologia subterràniaThis is the peer reviewed version of the following article: [Ding, D., Benson, D. A., Fernàndez‐Garcia, D., Henri, C. V., Hyndman, D. W., Phanikumar, M. S., & Bolster, D. (2017). Elimination of the reaction rate “scale effect”: Application of the Lagrangian reactive particle‐tracking method to simulate mixing‐limited, field‐scale biodegradation at the Schoolcraft (MI, USA) site. Water Resources Research, 53, 10,411–10,432. https://doi.org/10.1002/2017WR021103], which has been published in final form at https://doi.org/10.1002/2017WR021103. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Self-Archiving.Measured (or empirically fitted) reaction rates at groundwater remediation sites are typically much lower than those found in the same material at the batch or laboratory scale. The reduced rates are commonly attributed to poorer mixing at the larger scales. A variety of methods have been proposed to account for this scaling effect in reactive transport. In this study, we use the Lagrangian particle-tracking and reaction (PTR) method to simulate a field bioremediation experiment at the Schoolcraft, MI site. A denitrifying bacterium, Pseudomonas Stutzeri strain KC (KC), was injected to the aquifer, along with sufficient substrate, to degrade the contaminant, carbon tetrachloride (CT), under anaerobic conditions. The PTR method simulates chemical reactions through probabilistic rules of particle collisions, interactions, and transformations to address the scale effect (lower apparent reaction rates for each level of upscaling, from batch to column to field scale). In contrast to a prior Eulerian reaction model, the PTR method is able to match the field-scale experiment using the rate coefficients obtained from batch experiments.Peer Reviewed20172017-12-0120182018-03-20journal articlehttp://purl.org/coar/resource_type/c_6501AMhttp://purl.org/coar/version/c_ab4af688f83e57aainfo:eu-repo/semantics/articleapplication/pdfhttps://hdl.handle.net/2117/115474https://dx.doi.org/10.1002/2017WR021103reponame:UPCommons. Portal del coneixement obert de la UPCinstname:Universitat Politècnica de Catalunya (UPC)Inglésengopen accesshttp://purl.org/coar/access_right/c_abf2info:eu-repo/semantics/openAccessoai:upcommons.upc.edu:2117/1154742026-05-27T15:37:01Z
dc.title.none.fl_str_mv Elimination of the reaction rate 'scale effect': application of the Lagrangian reactive particle-tracking method to simulate mixing-limited, field-scale biodegradation at the Schoolcraft (MI, USA) site
title Elimination of the reaction rate 'scale effect': application of the Lagrangian reactive particle-tracking method to simulate mixing-limited, field-scale biodegradation at the Schoolcraft (MI, USA) site
spellingShingle Elimination of the reaction rate 'scale effect': application of the Lagrangian reactive particle-tracking method to simulate mixing-limited, field-scale biodegradation at the Schoolcraft (MI, USA) site
Dong, Ding
Bioremediation
Bioremediation
Particle tracking
Reactive transport
Scale effect
Bioremediació
Àrees temàtiques de la UPC::Enginyeria civil::Geologia::Hidrologia subterrània
title_short Elimination of the reaction rate 'scale effect': application of the Lagrangian reactive particle-tracking method to simulate mixing-limited, field-scale biodegradation at the Schoolcraft (MI, USA) site
title_full Elimination of the reaction rate 'scale effect': application of the Lagrangian reactive particle-tracking method to simulate mixing-limited, field-scale biodegradation at the Schoolcraft (MI, USA) site
title_fullStr Elimination of the reaction rate 'scale effect': application of the Lagrangian reactive particle-tracking method to simulate mixing-limited, field-scale biodegradation at the Schoolcraft (MI, USA) site
title_full_unstemmed Elimination of the reaction rate 'scale effect': application of the Lagrangian reactive particle-tracking method to simulate mixing-limited, field-scale biodegradation at the Schoolcraft (MI, USA) site
title_sort Elimination of the reaction rate 'scale effect': application of the Lagrangian reactive particle-tracking method to simulate mixing-limited, field-scale biodegradation at the Schoolcraft (MI, USA) site
dc.creator.none.fl_str_mv Dong, Ding
Benson, David A.
Fernández García, Daniel|||0000-0002-4667-3003
Henri, Christopher Vincent
Hyndman, David W.
Phanikumar, Mantha S.
Bolster, Diogo
author Dong, Ding
author_facet Dong, Ding
Benson, David A.
Fernández García, Daniel|||0000-0002-4667-3003
Henri, Christopher Vincent
Hyndman, David W.
Phanikumar, Mantha S.
Bolster, Diogo
author_role author
author2 Benson, David A.
Fernández García, Daniel|||0000-0002-4667-3003
Henri, Christopher Vincent
Hyndman, David W.
Phanikumar, Mantha S.
Bolster, Diogo
author2_role author
author
author
author
author
author
dc.subject.none.fl_str_mv Bioremediation
Bioremediation
Particle tracking
Reactive transport
Scale effect
Bioremediació
Àrees temàtiques de la UPC::Enginyeria civil::Geologia::Hidrologia subterrània
topic Bioremediation
Bioremediation
Particle tracking
Reactive transport
Scale effect
Bioremediació
Àrees temàtiques de la UPC::Enginyeria civil::Geologia::Hidrologia subterrània
description This is the peer reviewed version of the following article: [Ding, D., Benson, D. A., Fernàndez‐Garcia, D., Henri, C. V., Hyndman, D. W., Phanikumar, M. S., & Bolster, D. (2017). Elimination of the reaction rate “scale effect”: Application of the Lagrangian reactive particle‐tracking method to simulate mixing‐limited, field‐scale biodegradation at the Schoolcraft (MI, USA) site. Water Resources Research, 53, 10,411–10,432. https://doi.org/10.1002/2017WR021103], which has been published in final form at https://doi.org/10.1002/2017WR021103. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Self-Archiving.
publishDate 2017
dc.date.none.fl_str_mv 2017
2017-12-01
2018
2018-03-20
dc.type.none.fl_str_mv journal article
http://purl.org/coar/resource_type/c_6501
AM
http://purl.org/coar/version/c_ab4af688f83e57aa
dc.type.openaire.fl_str_mv info:eu-repo/semantics/article
format article
dc.identifier.none.fl_str_mv https://hdl.handle.net/2117/115474
https://dx.doi.org/10.1002/2017WR021103
url https://hdl.handle.net/2117/115474
https://dx.doi.org/10.1002/2017WR021103
dc.language.none.fl_str_mv Inglés
eng
language_invalid_str_mv Inglés
language eng
dc.rights.none.fl_str_mv open access
http://purl.org/coar/access_right/c_abf2
dc.rights.openaire.fl_str_mv info:eu-repo/semantics/openAccess
rights_invalid_str_mv open access
http://purl.org/coar/access_right/c_abf2
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
dc.source.none.fl_str_mv reponame:UPCommons. Portal del coneixement obert de la UPC
instname:Universitat Politècnica de Catalunya (UPC)
instname_str Universitat Politècnica de Catalunya (UPC)
reponame_str UPCommons. Portal del coneixement obert de la UPC
collection UPCommons. Portal del coneixement obert de la UPC
repository.name.fl_str_mv
repository.mail.fl_str_mv
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score 15,300719

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