Vacancy patterning and patterning vacancies: controlled self-assembly of fullerenes on metal surfaces

A density functional theory study accounting for van der Waals interactions reveals the potential of metal surface vacancies as anchor points for the construction of user-defined 2D patterns of adsorbate molecules via a controlled self-assembly process. Vice versa, energetic criteria indicate the fo...

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Detalles Bibliográficos
Autores: Kaiser, Alexander, Viñes Solana, Francesc, Illas i Riera, Francesc, Ritter, Marcel, Hagelberg, Frank, Probst, Michael
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2014
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2445/165801
Acceso en línea:https://hdl.handle.net/2445/165801
Access Level:acceso abierto
Palabra clave:Ful·lerens
Teoria del funcional de densitat
Adsorció
Fullerenes
Density functionals
Adsorption
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spelling Vacancy patterning and patterning vacancies: controlled self-assembly of fullerenes on metal surfacesKaiser, AlexanderViñes Solana, FrancescIllas i Riera, FrancescRitter, MarcelHagelberg, FrankProbst, MichaelFul·lerensTeoria del funcional de densitatAdsorcióFullerenesDensity functionalsAdsorptionA density functional theory study accounting for van der Waals interactions reveals the potential of metal surface vacancies as anchor points for the construction of user-defined 2D patterns of adsorbate molecules via a controlled self-assembly process. Vice versa, energetic criteria indicate the formation of regular adsorbate-induced vacancies after adsorbate self-assembly on clean surfaces. These processes are exemplified by adsorbing C60 fullerene on Al(111), Au(111), and Be(0001) surfaces with and without single, triple, and septuple atom pits. An analysis of vacancy-adatom formation energetics precedes the study of the adsorption processes.Royal Society of Chemistry2020202020142020info:eu-repo/semantics/articleinfo:eu-repo/semantics/acceptedVersion9 p.application/pdfhttps://hdl.handle.net/2445/165801Articles publicats en revistes (Ciència dels Materials i Química Física)reponame:Recercat. Dipósit de la Recerca de Catalunyainstname:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)InglésVersió postprint del document publicat a: https://doi.org/10.1039/C4NR02717ENanoscale, 2014, vol. 6, num. 18, p. 10850-10858https://doi.org/10.1039/C4NR02717Einfo:eu-repo/grantAgreement/EC/H2020/633053(c) Kaiser, Alexander et al., 2014info:eu-repo/semantics/openAccessoai:recercat.cat:2445/1658012026-05-29T05:05:01Z
dc.title.none.fl_str_mv Vacancy patterning and patterning vacancies: controlled self-assembly of fullerenes on metal surfaces
title Vacancy patterning and patterning vacancies: controlled self-assembly of fullerenes on metal surfaces
spellingShingle Vacancy patterning and patterning vacancies: controlled self-assembly of fullerenes on metal surfaces
Kaiser, Alexander
Ful·lerens
Teoria del funcional de densitat
Adsorció
Fullerenes
Density functionals
Adsorption
title_short Vacancy patterning and patterning vacancies: controlled self-assembly of fullerenes on metal surfaces
title_full Vacancy patterning and patterning vacancies: controlled self-assembly of fullerenes on metal surfaces
title_fullStr Vacancy patterning and patterning vacancies: controlled self-assembly of fullerenes on metal surfaces
title_full_unstemmed Vacancy patterning and patterning vacancies: controlled self-assembly of fullerenes on metal surfaces
title_sort Vacancy patterning and patterning vacancies: controlled self-assembly of fullerenes on metal surfaces
dc.creator.none.fl_str_mv Kaiser, Alexander
Viñes Solana, Francesc
Illas i Riera, Francesc
Ritter, Marcel
Hagelberg, Frank
Probst, Michael
author Kaiser, Alexander
author_facet Kaiser, Alexander
Viñes Solana, Francesc
Illas i Riera, Francesc
Ritter, Marcel
Hagelberg, Frank
Probst, Michael
author_role author
author2 Viñes Solana, Francesc
Illas i Riera, Francesc
Ritter, Marcel
Hagelberg, Frank
Probst, Michael
author2_role author
author
author
author
author
dc.subject.none.fl_str_mv Ful·lerens
Teoria del funcional de densitat
Adsorció
Fullerenes
Density functionals
Adsorption
topic Ful·lerens
Teoria del funcional de densitat
Adsorció
Fullerenes
Density functionals
Adsorption
description A density functional theory study accounting for van der Waals interactions reveals the potential of metal surface vacancies as anchor points for the construction of user-defined 2D patterns of adsorbate molecules via a controlled self-assembly process. Vice versa, energetic criteria indicate the formation of regular adsorbate-induced vacancies after adsorbate self-assembly on clean surfaces. These processes are exemplified by adsorbing C60 fullerene on Al(111), Au(111), and Be(0001) surfaces with and without single, triple, and septuple atom pits. An analysis of vacancy-adatom formation energetics precedes the study of the adsorption processes.
publishDate 2014
dc.date.none.fl_str_mv 2014
2020
2020
2020
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/acceptedVersion
format article
status_str acceptedVersion
dc.identifier.none.fl_str_mv https://hdl.handle.net/2445/165801
url https://hdl.handle.net/2445/165801
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv Versió postprint del document publicat a: https://doi.org/10.1039/C4NR02717E
Nanoscale, 2014, vol. 6, num. 18, p. 10850-10858
https://doi.org/10.1039/C4NR02717E
info:eu-repo/grantAgreement/EC/H2020/633053
dc.rights.none.fl_str_mv (c) Kaiser, Alexander et al., 2014
info:eu-repo/semantics/openAccess
rights_invalid_str_mv (c) Kaiser, Alexander et al., 2014
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv 9 p.
application/pdf
dc.publisher.none.fl_str_mv Royal Society of Chemistry
publisher.none.fl_str_mv Royal Society of Chemistry
dc.source.none.fl_str_mv Articles publicats en revistes (Ciència dels Materials i Química Física)
reponame:Recercat. Dipósit de la Recerca de Catalunya
instname:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
instname_str Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
reponame_str Recercat. Dipósit de la Recerca de Catalunya
collection Recercat. Dipósit de la Recerca de Catalunya
repository.name.fl_str_mv
repository.mail.fl_str_mv
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score 15,811543

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