Polymorphic phase boundary in piezoelectric oxides

The design of phase boundaries has now become a consolidated strategy to improve the functional properties of piezoelectric oxides because of the unique properties that may be obtained in their vicinity. In particular, polymorphic phase boundaries (PPBs) have attracted significant interest in recent...

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Detalles Bibliográficos
Autores: García García, José Eduardo|||0000-0002-1232-1739, Rubio Marcos, Fernando
Tipo de recurso: artículo
Fecha de publicación:2020
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/183124
Acceso en línea:https://hdl.handle.net/2117/183124
https://dx.doi.org/10.1063/5.0002983
Access Level:acceso abierto
Palabra clave:Oxides
Ceramics
X-rays - Diffraction
Polymorphism (Crystallography)
Perovskite
Phase transformations (Statistical physics)
Polycrystals
Piezoelectric materials
X-ray diffraction
Ferroelectric materials
Polymorphism
Perovskites
Phase transitions
Polycrystalline material
Òxids
Ceràmica industrial
Raigs X -- Difracció
Polimorfisme (Cristal·lografia)
Perovskita
Transicions de fase (Física estadística)
Policristal·lins
Àrees temàtiques de la UPC::Física
Descripción
Sumario:The design of phase boundaries has now become a consolidated strategy to improve the functional properties of piezoelectric oxides because of the unique properties that may be obtained in their vicinity. In particular, polymorphic phase boundaries (PPBs) have attracted significant interest in recent years because they represent a significant breakthrough in terms of enhanced piezoelectric activity of lead-free piezoelectric oxides. PPBs are temperature-driven phase transitions where both intrinsic and extrinsic contributions maximize, thereby enhancing the macroscopic properties of piezoelectric materials. This tutorial discusses potassium–sodium–niobate-based systems as model materials to reveal some of the most relevant advances in the design of PPBs through compositional modifications. We focus on how PPBs can be modulated by engineered doping and also discuss the direct relation between PPBs and the enhancement of piezoelectric activity. Finally, we briefly describe the main experimental techniques for detecting PPBs.