UO2 as new filling material for cesium retention in high-level nuclear waste repositories

Depleted uranium dioxide has been proposed as an inert material to fill spent nuclear fuel canisters in geological repositories. Sorption capacity of this material to retain radionuclides released from the fuel was determined. Radiocesium is one of the radionuclides of concern in case of a nuclear a...

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Detalles Bibliográficos
Autores: Martínez Torrents, Albert, Gimenez, Javier, Pablo Ribas, Joan de|||0000-0001-9538-7321, Casas Pons, Ignasi|||0000-0002-5419-1645
Tipo de recurso: artículo
Fecha de publicación:2015
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/83067
Acceso en línea:https://hdl.handle.net/2117/83067
https://dx.doi.org/10.1089/ees.2015.0129
Access Level:acceso abierto
Palabra clave:Spent reactor fuels--Storage
depleted UO2
Langmuir isotherm
radiocesium
spent fuel canister
UO2 sorption
uranium-oxides
mobilization
sediments
transport
colloids
Combustibles nuclears gastats Emmagatzematge
Àrees temàtiques de la UPC::Enginyeria química
Descripción
Sumario:Depleted uranium dioxide has been proposed as an inert material to fill spent nuclear fuel canisters in geological repositories. Sorption capacity of this material to retain radionuclides released from the fuel was determined. Radiocesium is one of the radionuclides of concern in case of a nuclear accident or in a high-level nuclear waste repository and is highly mobile in aquatic systems. Results obtained in this work show that sorption of cesium on UO2 is a fast process (the equilibrium is reached in less than 1h at pH 9).