Anomalous Size Dependence in the Melting Temperatures of Free Sodium Clusters: An Explanation for the Calorimetry Experiments

Producción Científica

Bibliographic Details
Authors: López Rodríguez, José Manuel, Aguado Rodríguez, Andrés
Format: article
Publication Date:2005
Country:España
Institution:Universidad de Valladolid
Repository:UVaDOC. Repositorio Documental de la Universidad de Valladolid
OAI Identifier:oai:uvadoc.uva.es:10324/2445
Online Access:https://doi.org/10.1103/PhysRevLett.94.233401
http://uvadoc.uva.es/handle/10324/2445
Access Level:Open access
Keyword:Calorímetros y calorimetría
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spelling Anomalous Size Dependence in the Melting Temperatures of Free Sodium Clusters: An Explanation for the Calorimetry ExperimentsLópez Rodríguez, José ManuelAguado Rodríguez, AndrésCalorímetros y calorimetríaProducción CientíficaThe meltinglike transition in unsupported NaN clusters (N=55, 92, 147, 181, 189, 215, 249, 271, 281 and 299) is studied by first-principles isokinetic molecular dynamics simulations. The irregular size dependence of the melting temperatures Tm observed in the calorimetry experiments of Schmidt et al. [ Nature (London) 393 238 (1998)] is quantitatively reproduced. We demonstrate that structural effects alone can explain all broad features of experimental observations. Specifically, maxima in Tm(N) correlate with high surface stability and with structural features such as a high compactness degree.The American Physical Society2005info:eu-repo/semantics/articleapplication/pdfhttps://doi.org/10.1103/PhysRevLett.94.233401http://uvadoc.uva.es/handle/10324/2445reponame:UVaDOC. Repositorio Documental de la Universidad de Valladolidinstname:Universidad de ValladolidIngléshttp://link.aps.org/doi/10.1103/PhysRevLett.94.233401info:eu-repo/semantics/openAccesshttp://creativecommons.org/licenses/by-nc-nd/3.0/es/oai:uvadoc.uva.es:10324/24452026-06-13T12:44:47Z
dc.title.none.fl_str_mv Anomalous Size Dependence in the Melting Temperatures of Free Sodium Clusters: An Explanation for the Calorimetry Experiments
title Anomalous Size Dependence in the Melting Temperatures of Free Sodium Clusters: An Explanation for the Calorimetry Experiments
spellingShingle Anomalous Size Dependence in the Melting Temperatures of Free Sodium Clusters: An Explanation for the Calorimetry Experiments
López Rodríguez, José Manuel
Calorímetros y calorimetría
title_short Anomalous Size Dependence in the Melting Temperatures of Free Sodium Clusters: An Explanation for the Calorimetry Experiments
title_full Anomalous Size Dependence in the Melting Temperatures of Free Sodium Clusters: An Explanation for the Calorimetry Experiments
title_fullStr Anomalous Size Dependence in the Melting Temperatures of Free Sodium Clusters: An Explanation for the Calorimetry Experiments
title_full_unstemmed Anomalous Size Dependence in the Melting Temperatures of Free Sodium Clusters: An Explanation for the Calorimetry Experiments
title_sort Anomalous Size Dependence in the Melting Temperatures of Free Sodium Clusters: An Explanation for the Calorimetry Experiments
dc.creator.none.fl_str_mv López Rodríguez, José Manuel
Aguado Rodríguez, Andrés
author López Rodríguez, José Manuel
author_facet López Rodríguez, José Manuel
Aguado Rodríguez, Andrés
author_role author
author2 Aguado Rodríguez, Andrés
author2_role author
dc.subject.none.fl_str_mv Calorímetros y calorimetría
topic Calorímetros y calorimetría
description Producción Científica
publishDate 2005
dc.date.none.fl_str_mv 2005
dc.type.none.fl_str_mv info:eu-repo/semantics/article
format article
dc.identifier.none.fl_str_mv https://doi.org/10.1103/PhysRevLett.94.233401
http://uvadoc.uva.es/handle/10324/2445
url https://doi.org/10.1103/PhysRevLett.94.233401
http://uvadoc.uva.es/handle/10324/2445
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv http://link.aps.org/doi/10.1103/PhysRevLett.94.233401
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
http://creativecommons.org/licenses/by-nc-nd/3.0/es/
eu_rights_str_mv openAccess
rights_invalid_str_mv http://creativecommons.org/licenses/by-nc-nd/3.0/es/
dc.format.none.fl_str_mv application/pdf
dc.publisher.none.fl_str_mv The American Physical Society
publisher.none.fl_str_mv The American Physical Society
dc.source.none.fl_str_mv reponame:UVaDOC. Repositorio Documental de la Universidad de Valladolid
instname:Universidad de Valladolid
instname_str Universidad de Valladolid
reponame_str UVaDOC. Repositorio Documental de la Universidad de Valladolid
collection UVaDOC. Repositorio Documental de la Universidad de Valladolid
repository.name.fl_str_mv
repository.mail.fl_str_mv
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score 15.301603

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