Understanding the effect of the nature of the nucleobase in the loops on the stability of the i-motif structure

The nature and length of loops connecting cytosine tracts in i-motif structures may affect their stability. In this work, the influence of the nature of the nucleobases located in two of the loops of an intramolecular i-motif is studied using spectroscopy, separation techniques, and multivariate dat...

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Detalles Bibliográficos
Autores: Benabou Zdaou, Sanae, Garavís, Miguel, Lyonnais, Sébastien, Eritja i Casadellà, Ramon, González, Carlos, Gargallo Gómez, Raimundo
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2016
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2445/127915
Acceso en línea:https://hdl.handle.net/2445/127915
Access Level:acceso abierto
Palabra clave:ADN
Espectroscòpia de ressonància magnètica nuclear
Cromatografia de permeació per gel
Electroforesi
DNA
Nuclear magnetic resonance spectroscopy
Gel permeation chromatography
Electrophoresis
Descripción
Sumario:The nature and length of loops connecting cytosine tracts in i-motif structures may affect their stability. In this work, the influence of the nature of the nucleobases located in two of the loops of an intramolecular i-motif is studied using spectroscopy, separation techniques, and multivariate data analysis. Insertion of bases other than thymine induces an additional acid-base equilibrium with pKa~4.5. The presence of two guanine bases in the loops, placed opposite to each other, decreases the thermal stability of the structure. In contrast, thymine and cytosine bases in these positions stabilize the structure