A generalized approach for evaluating the mechanical properties of polymer nanocomposites reinforced with spherical fillers

This article belongs to the Special Issue Polymer Nanocomposites: Preparation, Characterisation and Applications.

Detalles Bibliográficos
Autores: Martínez-García, Julio César, Serraïma-Ferrer, Alexandre, Lopeandía, Aitor, Lattuada, Marco, Sapkota, Janak, Rodríguez-Viejo, Javier
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2021
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/253108
Acceso en línea:http://hdl.handle.net/10261/253108
Access Level:acceso abierto
Palabra clave:Percolation threshold
Polymer nanocomposites
Mechanical reinforcement
Interphase modeling
Nanocomposites
Interphase
Spherical fillers
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spelling A generalized approach for evaluating the mechanical properties of polymer nanocomposites reinforced with spherical fillersMartínez-García, Julio CésarSerraïma-Ferrer, AlexandreLopeandía, AitorLattuada, MarcoSapkota, JanakRodríguez-Viejo, JavierPercolation thresholdPolymer nanocompositesMechanical reinforcementInterphase modelingNanocompositesInterphaseSpherical fillersThis article belongs to the Special Issue Polymer Nanocomposites: Preparation, Characterisation and Applications.In this work, the effective mechanical reinforcement of polymeric nanocomposites containing spherical particle fillers is predicted based on a generalized analytical three-phase-series-parallel model, considering the concepts of percolation and the interfacial glassy region. While the concept of percolation is solely taken as a contribution of the filler-network, we herein show that the glassy interphase between filler and matrix, which is often in the nanometers range, is also to be considered while interpreting enhanced mechanical properties of particulate filled polymeric nanocomposites. To demonstrate the relevance of the proposed generalized equation, we have fitted several experimental results which show a good agreement with theoretical predictions. Thus, the approach presented here can be valuable to elucidate new possible conceptual routes for the creation of new materials with fundamental technological applications and can open a new research avenue for future studies.This research was funded by the Catalan government within the Beatriu de Pinos program, grant number NB615798.Peer reviewedMultidisciplinary Digital Publishing InstituteGeneralitat de CatalunyaConsejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]202120212021info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501Publisher's versioninfo:eu-repo/semantics/publishedVersionhttp://hdl.handle.net/10261/253108reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Ingléshttps://doi.org/10.3390/nano11040830Síinfo:eu-repo/semantics/openAccessoai:digital.csic.es:10261/2531082026-05-22T06:33:51Z
dc.title.none.fl_str_mv A generalized approach for evaluating the mechanical properties of polymer nanocomposites reinforced with spherical fillers
title A generalized approach for evaluating the mechanical properties of polymer nanocomposites reinforced with spherical fillers
spellingShingle A generalized approach for evaluating the mechanical properties of polymer nanocomposites reinforced with spherical fillers
Martínez-García, Julio César
Percolation threshold
Polymer nanocomposites
Mechanical reinforcement
Interphase modeling
Nanocomposites
Interphase
Spherical fillers
title_short A generalized approach for evaluating the mechanical properties of polymer nanocomposites reinforced with spherical fillers
title_full A generalized approach for evaluating the mechanical properties of polymer nanocomposites reinforced with spherical fillers
title_fullStr A generalized approach for evaluating the mechanical properties of polymer nanocomposites reinforced with spherical fillers
title_full_unstemmed A generalized approach for evaluating the mechanical properties of polymer nanocomposites reinforced with spherical fillers
title_sort A generalized approach for evaluating the mechanical properties of polymer nanocomposites reinforced with spherical fillers
dc.creator.none.fl_str_mv Martínez-García, Julio César
Serraïma-Ferrer, Alexandre
Lopeandía, Aitor
Lattuada, Marco
Sapkota, Janak
Rodríguez-Viejo, Javier
author Martínez-García, Julio César
author_facet Martínez-García, Julio César
Serraïma-Ferrer, Alexandre
Lopeandía, Aitor
Lattuada, Marco
Sapkota, Janak
Rodríguez-Viejo, Javier
author_role author
author2 Serraïma-Ferrer, Alexandre
Lopeandía, Aitor
Lattuada, Marco
Sapkota, Janak
Rodríguez-Viejo, Javier
author2_role author
author
author
author
author
dc.contributor.none.fl_str_mv Generalitat de Catalunya
Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]
dc.subject.none.fl_str_mv Percolation threshold
Polymer nanocomposites
Mechanical reinforcement
Interphase modeling
Nanocomposites
Interphase
Spherical fillers
topic Percolation threshold
Polymer nanocomposites
Mechanical reinforcement
Interphase modeling
Nanocomposites
Interphase
Spherical fillers
description This article belongs to the Special Issue Polymer Nanocomposites: Preparation, Characterisation and Applications.
publishDate 2021
dc.date.none.fl_str_mv 2021
2021
2021
dc.type.none.fl_str_mv info:eu-repo/semantics/article
http://purl.org/coar/resource_type/c_6501
Publisher's version
info:eu-repo/semantics/publishedVersion
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/10261/253108
url http://hdl.handle.net/10261/253108
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv https://doi.org/10.3390/nano11040830
Sí
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.publisher.none.fl_str_mv Multidisciplinary Digital Publishing Institute
publisher.none.fl_str_mv Multidisciplinary Digital Publishing Institute
dc.source.none.fl_str_mv reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC
instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str DIGITAL.CSIC. Repositorio Institucional del CSIC
collection DIGITAL.CSIC. Repositorio Institucional del CSIC
repository.name.fl_str_mv
repository.mail.fl_str_mv
_version_ 1869412601805406208
score 15,811543

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