A new route of synthesis of Na-Mica-4 from sodalite

Synthesis of Na-Mica-4 has been achieved by a ``mix and calcine¿¿ method using sodalite and magnesium fluoride as the only precursors. Previous research found sodalite as a key intermediate reaction product in the formation of Na-Mica-4 when the NaCl melt method was employed. Similarities in structu...

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Detalles Bibliográficos
Autores: Naranjo Muñoz, Moisés, Castro Arroyo, Miguel Ángel, Cota Reguero, Agustín, Pavón González, Esperanza, Pazos Zarama, Mery Carolina, Alba Carranza, María Dolores
Tipo de recurso: artículo
Estado:Versión enviada para evaluación y publicación
Fecha de publicación:2014
País:España
Institución:Universidad de Sevilla (US)
Repositorio:idUS. Depósito de Investigación de la Universidad de Sevilla
OAI Identifier:oai:idus.us.es:11441/66997
Acceso en línea:http://hdl.handle.net/11441/66997
https://doi.org/10.1016/j.micromeso.2013.12.004
Access Level:acceso abierto
Palabra clave:Rheology
XRD
MAS NMR
Sodalite
Brittle micas
Descripción
Sumario:Synthesis of Na-Mica-4 has been achieved by a ``mix and calcine¿¿ method using sodalite and magnesium fluoride as the only precursors. Previous research found sodalite as a key intermediate reaction product in the formation of Na-Mica-4 when the NaCl melt method was employed. Similarities in structure, chemical composition and cation distribution in products using the proposed method and the NaCl melt method are described and suggest that Na-Mica-4 is a very stable product. The use of sodalite as precursor provokes microporous formation in the final mica. The absence of excess Na leads to a lower particle size and to the presence of less impurity in the calcined product. Different sodalites could be used in the synthesis of different Na-Mica-4 with presumably different physicochemical properties