An iron catalyst for oxidation of alkyl C-H bonds showing enhanced selectivity for methylenic sites

Many are called but few are chosen: A nonheme iron complex catalyzes the oxidation of alkyl C[BOND]H bonds by using H2O2 as the oxidant, showing an enhanced selectivity for secondary over tertiary C[BOND]H bonds (see scheme)

Detalhes bibliográficos
Autores: Prat Casellas, Irene, Gómez Martín, Laura, Canta i Roldós, Mercè, Ribas Salamaña, Xavi, Costas Salgueiro, Miquel
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2013
País:España
Recursos:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositório:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:10256/12260
Acesso em linha:http://hdl.handle.net/10256/12260
Access Level:Acesso embargado
Palavra-chave:Catàlisi
Catalysis
Catàlisi homogènia
Homogeneous catalysis
Aigua oxigenada
Hydrogen peroxide
Ferro
Iron
Catalitzadors de ferro
Iron catalysts
Descrição
Resumo:Many are called but few are chosen: A nonheme iron complex catalyzes the oxidation of alkyl C[BOND]H bonds by using H2O2 as the oxidant, showing an enhanced selectivity for secondary over tertiary C[BOND]H bonds (see scheme)