Improving the degradation of low concentration of microcystin-LR with PEM 2 electrolyzers and photo-electrolyzers

In this work, the performances of two electrochemical cells, a conventional liquid-electrolyte electrolyzer (LEE) and a solid-electrolyte electrolyzer (SEE) were compared for the treatment of two real water matrixes polluted with microcystin-LR at trace concentrations. The first consists of single-c...

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Detalles Bibliográficos
Autores: Souza, Fernanda L., Sáez Jiménez, Cristina, Cañizares Cañizares, Pablo, Rodrigo Rodrigo, Manuel Andrés
Tipo de recurso: artículo
Fecha de publicación:2021
País:España
Institución:Universidad de Castilla-La Mancha
Repositorio:RUIdeRA. Repositorio Institucional de la UCLM
OAI Identifier:oai:ruidera.uclm.es:10578/29140
Acceso en línea:http://hdl.handle.net/10578/29140
Access Level:acceso abierto
Palabra clave:Electroquímica
Ingeniería química
Descripción
Sumario:In this work, the performances of two electrochemical cells, a conventional liquid-electrolyte electrolyzer (LEE) and a solid-electrolyte electrolyzer (SEE) were compared for the treatment of two real water matrixes polluted with microcystin-LR at trace concentrations. The first consists of single-compartment flow cell, while the second consists of membrane-electrode assembly flow cell. Both cells can attain the removal of the microcystin, although the toxin degradation was more efficient in the SEE, for both water matrixes assessed, decreasing the initial concentration by 3-logs and achieving in short treatment times concentrations below the guidelines of the World Health Organization (WHO) for drinking water. Irradiation of UVC improves results reached by the electrochemical technologies, although in lower extension than initially expected. The great performance of SEE reactor is attributed to a more suitable production of oxidants and a lower operation-dependence with respect to the water matrix conductivity. This cell can remove pollutants also faster than the single photolysis and, in comparing its performance with the other technologies assessed in this work, it is the best choice requiring the less time and energy to meet the WHO standards, without being necessary the coupling with photolysis.