Mesoporous Matrices as Hosts for Metal Halide Perovskite Nanocrystals

Several works have recently demonstrated that perovskite nanocrystals can be controllably formed within a variety of porous matrices employing diverse synthetic strategies. By means of the fine tuning of the pore size distribution, the thickness and composition of the walls, the geometry of the void...

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Detalles Bibliográficos
Autores: Rubino, Andrea, Calió, Laura, García-Bennett, A., Calvo, Mauricio E., Míguez, Hernán
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2020
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/216685
Acceso en línea:http://hdl.handle.net/10261/216685
Access Level:acceso abierto
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spelling Mesoporous Matrices as Hosts for Metal Halide Perovskite NanocrystalsRubino, AndreaCalió, LauraGarcía-Bennett, A.Calvo, Mauricio E.Míguez, HernánSeveral works have recently demonstrated that perovskite nanocrystals can be controllably formed within a variety of porous matrices employing diverse synthetic strategies. By means of the fine tuning of the pore size distribution, the thickness and composition of the walls, the geometry of the void network and its topology, strict control over the structural and morphological parameters of the hosted semiconductor can be achieved, determining its optical absorption and emission properties. Furthermore, porous hosts provide the guest semiconductor with enhanced stability and versatility in terms of processing, which favors its integration in devices. This article provides a comprehensive review of the different approaches proposed, as well as a discussion on the relevance they may have for the development of nanostructured perovskite¿based optoelectronics. A critical assessment of the optical quality of the hybrid perovskite nanomaterials so obtained is presented, as well as an analysis of the fundamental and applied aspects of the nanocrystal¿matrix interaction and a projected prospect of their impact in the fields of artificial lighting and renewable energy.Wiley-BlackwellConsejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]2020202020202020info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501Postprintinfo:eu-repo/semantics/acceptedVersionhttp://hdl.handle.net/10261/216685reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Ingléshttp://dx.doi.org/10.1002/adom.201901868Síinfo:eu-repo/semantics/openAccessoai:digital.csic.es:10261/2166852026-05-22T06:33:51Z
dc.title.none.fl_str_mv Mesoporous Matrices as Hosts for Metal Halide Perovskite Nanocrystals
title Mesoporous Matrices as Hosts for Metal Halide Perovskite Nanocrystals
spellingShingle Mesoporous Matrices as Hosts for Metal Halide Perovskite Nanocrystals
Rubino, Andrea
title_short Mesoporous Matrices as Hosts for Metal Halide Perovskite Nanocrystals
title_full Mesoporous Matrices as Hosts for Metal Halide Perovskite Nanocrystals
title_fullStr Mesoporous Matrices as Hosts for Metal Halide Perovskite Nanocrystals
title_full_unstemmed Mesoporous Matrices as Hosts for Metal Halide Perovskite Nanocrystals
title_sort Mesoporous Matrices as Hosts for Metal Halide Perovskite Nanocrystals
dc.creator.none.fl_str_mv Rubino, Andrea
Calió, Laura
García-Bennett, A.
Calvo, Mauricio E.
Míguez, Hernán
author Rubino, Andrea
author_facet Rubino, Andrea
Calió, Laura
García-Bennett, A.
Calvo, Mauricio E.
Míguez, Hernán
author_role author
author2 Calió, Laura
García-Bennett, A.
Calvo, Mauricio E.
Míguez, Hernán
author2_role author
author
author
author
dc.contributor.none.fl_str_mv Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]
description Several works have recently demonstrated that perovskite nanocrystals can be controllably formed within a variety of porous matrices employing diverse synthetic strategies. By means of the fine tuning of the pore size distribution, the thickness and composition of the walls, the geometry of the void network and its topology, strict control over the structural and morphological parameters of the hosted semiconductor can be achieved, determining its optical absorption and emission properties. Furthermore, porous hosts provide the guest semiconductor with enhanced stability and versatility in terms of processing, which favors its integration in devices. This article provides a comprehensive review of the different approaches proposed, as well as a discussion on the relevance they may have for the development of nanostructured perovskite¿based optoelectronics. A critical assessment of the optical quality of the hybrid perovskite nanomaterials so obtained is presented, as well as an analysis of the fundamental and applied aspects of the nanocrystal¿matrix interaction and a projected prospect of their impact in the fields of artificial lighting and renewable energy.
publishDate 2020
dc.date.none.fl_str_mv 2020
2020
2020
2020
dc.type.none.fl_str_mv info:eu-repo/semantics/article
http://purl.org/coar/resource_type/c_6501
Postprint
info:eu-repo/semantics/acceptedVersion
format article
status_str acceptedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/10261/216685
url http://hdl.handle.net/10261/216685
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv http://dx.doi.org/10.1002/adom.201901868
Sí
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.publisher.none.fl_str_mv Wiley-Blackwell
publisher.none.fl_str_mv Wiley-Blackwell
dc.source.none.fl_str_mv reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC
instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str DIGITAL.CSIC. Repositorio Institucional del CSIC
collection DIGITAL.CSIC. Repositorio Institucional del CSIC
repository.name.fl_str_mv
repository.mail.fl_str_mv
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score 15,811543

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