Dimethylglyoxime modified screen-printed electrodes for nickel determination

This work reports the development of a dimethylglyoxime (DMG) modified sensor in which the complexing agent was successfully immobilized by drop-casting onto a screen-printed carbon electrode support (SPCE). The experimental conditions for the preparation of the DMG-SPCE sensor were optimized by mea...

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Detalles Bibliográficos
Autores: Rosal Soria, Miguel, Cetó Alseda, Xavier, Serrano i Plana, Núria, Ariño Blasco, Cristina, Esteban i Cortada, Miquel, Díaz Cruz, José Manuel
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2019
País:España
Institución:Universidad de Barcelona
Repositorio:Dipòsit Digital de la UB
OAI Identifier:oai:diposit.ub.edu:2445/139417
Acceso en línea:https://hdl.handle.net/2445/139417
Access Level:acceso abierto
Palabra clave:Níquel
Voltametria
Anàlisi electroquímica
Electroquímica
Nickel
Voltammetry
Electrochemical analysis
Electrochemistry
Descripción
Sumario:This work reports the development of a dimethylglyoxime (DMG) modified sensor in which the complexing agent was successfully immobilized by drop-casting onto a screen-printed carbon electrode support (SPCE). The experimental conditions for the preparation of the DMG-SPCE sensor were optimized by means of a D-optimal design, and the built sensors were analytically evaluated for the determination of Ni(II) by adsorptive stripping voltammetry (AdSV). Its analytical performance suggests its suitability for the determination of Ni(II)-ions by AdSV at concentration levels of μg L-1 (LOD of 2.3 μg L-1, linear range from 7.6 to 200 μg L-1). Finally, the applicability of the developed sensor was assessed by the determination of trace levels of Ni(II) by AdSV in a wastewater reference material with a very high reproducibility (0.005 %) and good trueness (0.1 %).