Direct Conversion of Syngas to Higher Alcohols via Tandem Integration of Fischer-Tropsch Synthesis and Reductive Hydroformylation

[EN] The selective conversion of syngas to higher alcohols is an attractive albeit elusive route in the quest for effective production of chemicals from alternative carbon resources. We report the tandem integration of solid cobalt Fischer-Tropsch and molecular hydroformylation catalysts in a one-po...

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Detalles Bibliográficos
Autores: Jeske, Kai, Rösler, Thorsten, Maurice Belleflamme, Nico Fischer, Michael Claeys, Walter Leitner, Andreas J. Vorholt, Ródenas Torralba, Tania, Prieto González, Gonzalo|||0000-0002-0956-3040
Tipo de recurso: artículo
Fecha de publicación:2022
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/193570
Acceso en línea:https://riunet.upv.es/handle/10251/193570
Access Level:acceso abierto
Palabra clave:Cascade Reactions
Higher Oxygenates
Plasticizer Alcohols
Syngas Conversion
Tandem Catalysis
Descripción
Sumario:[EN] The selective conversion of syngas to higher alcohols is an attractive albeit elusive route in the quest for effective production of chemicals from alternative carbon resources. We report the tandem integration of solid cobalt Fischer-Tropsch and molecular hydroformylation catalysts in a one-pot slurry-phase process. Unprecedented selectivities (>50 wt %) to C2+ alcohols are achieved at CO conversion levels >70 %, alongside negligible CO2 side-production. The efficient overall transformation is enabled by catalyst engineering, bridging gaps in operation temperature and intrinsic selectivity which have classically precluded integration of these reactions in a single conversion step. Swift capture of 1-olefin Fischer-Tropsch primary products by the molecular hydroformylation catalyst, presumably within the pores of the solid catalyst is key for high alcohol selectivity. The results underscore that controlled cooperation between solid aggregate and soluble molecular metal catalysts, which pertain to traditionally dichotomic realms of heterogeneous and homogeneous catalysis, is a promising blueprint toward selective conversion processes.