On the impact of excess diesel NOX emissions upon NO2 pollution in a compact city

NOX emissions from diesel light-duty-vehicles (LDV) largely exceed the Euro emission standards in real-world driving conditions. Recent studies have quantified their impact upon air quality and human health primarily based on air quality models at mesoscale and large-scale resolutions. Here, we show...

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Detalles Bibliográficos
Autores: Benavides, Jaime, Guevara Vilardell, Marc|||0000-0001-9727-8583, Snyde, Michelle G, Rodríguez Rey, Daniel, Soret, Albert|||0000-0002-1962-2972, Pérez García-Pando, Carlos|||0000-0002-4456-0697, Jorba Casellas, Oriol|||0000-0001-5872-0244
Tipo de recurso: artículo
Fecha de publicación:2021
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/340453
Acceso en línea:https://hdl.handle.net/2117/340453
https://dx.doi.org/10.1088/1748-9326/abd5dd
Access Level:acceso abierto
Palabra clave:Diesel automobiles
Air quality
Model resolution
Light duty vehicles
Excess diesel NOX emissions
NO2 concentrations
NO2 exposure
Motors dièsel -- Gas d'escapament
Qualitat ambiental
Aire -- Contaminació
Àrees temàtiques de la UPC::Desenvolupament humà i sostenible::Degradació ambiental::Contaminació atmosfèrica
Descripción
Sumario:NOX emissions from diesel light-duty-vehicles (LDV) largely exceed the Euro emission standards in real-world driving conditions. Recent studies have quantified their impact upon air quality and human health primarily based on air quality models at mesoscale and large-scale resolutions. Here, we show that these approaches can significantly underestimate the impact of diesel LDV excess NOX emissions upon NO2 pollution in cities, particularly in the more compact and heavily trafficked ones. We compare an air quality mesoscale model at both 4 and 1 km resolution with a street-scale model in Barcelona, a compact city where the EU annual NO2 limits are repeatedly exceeded and a large share of passenger cars are diesel (65%). We compare consistently two emissions scenarios: a business-as-usual scenario where diesel LDV emit NOX in excess, and a counterfactual standard limits scenario where emissions are compliant with the Euro emission standards. We first show that in contrast to the mesoscale model, the street scale model is able to largely represent the observed NO2 concentration gradients between traffic and background stations in the city. In a second step, we find that the mesoscale model strongly underestimates the impact of diesel LDV excess NOX emissions upon NO2 pollution both in absolute terms (by 38%–48%) and relative terms (by 10%–35%). We argue that such underestimated impacts should be considered when assessing NOX excess emissions by LDV in cities. Using the street scale model, we find that diesel LDV excess NOX emissions are associated with about 20% of NO2 levels in the city, contributing substantially to an increased number of citizens exposed to high NO2 pollution in Barcelona.